中国某重污染地区土壤中重金属的人为增加

IF 3.6 4区 环境科学与生态学 Q2 BIOCHEMISTRY & MOLECULAR BIOLOGY
Jiaxin Wang, Qingye Hou, Zhongfang Yang, Tao Yu, Riyang Wen
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引用次数: 0

摘要

评价重污染地区人为活动引起的土壤重金属浓度变化具有重要意义。土壤重金属污染程度的评价主要采用不同指标、不同标准和不同参考元素。然而,这些方法不能用于评价人为活动造成的重金属污染程度。本研究选取中国株洲为污染区,选取与株洲地质和气候条件相似的岳阳为背景区。污染区土壤垂直剖面As (6.6 ~ 23.6 mg/kg)、Cd (0.125 ~ 0.757 mg/kg)、Cu (33 ~ 75 mg/kg)、Hg (0.032 ~ 0.202 mg/kg)、Pb (17 ~ 108 mg/kg)、Zn (74 ~ 122 mg/kg)浓度均高于背景区(分别为1.7 ~ 20.7、0.085 ~ 0.210、21 ~ 47、0.030 ~ 0.105、17 ~ 38、32 ~ 88 mg/kg)。K2O/Al2O3、SiO2/Al2O3、风化淋滤系数ba差异不大,说明两区土壤风化程度相近。土壤的风化程度决定了重金属和参考元素的地球化学行为。根据背景区土壤剖面重金属浓度与有机碳、K2O/Al2O3、SiO2/Al2O3的预测模型,描述了污染区表层土壤重金属浓度的上升趋势。表层土壤重金属浓度受人为活动影响明显。本研究为评价人类活动对土壤重金属的影响提供了一个案例研究。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Anthropogenic increase of heavy metals in soil from a heavily contaminated area of China
Evaluating the variation in heavy metal concentrations in soil caused by anthropogenic activities in heavily contaminated areas is of great significance. The degree of heavy metal pollution in soil is primarily assessed by different indices with different standards and reference elements. However, these methods cannot be used to evaluate the degree of heavy metal pollution caused by anthropogenic activities. In this study, Zhuzhou, China was selected as the contaminated area, and Yueyang, China was selected as the background area, where geological and climatic conditions are similar to those of Zhuzhou, China. The concentrations of As (6.6–23.6 mg/kg), Cd (0.125–0.757 mg/kg), Cu (33–75 mg/kg), Hg (0.032–0.202 mg/kg), Pb (17–108 mg/kg), and Zn (74–122 mg/kg) in the vertical soil profiles in the contaminated area were higher than those in the background area (ranging 1.7–20.7, 0.085–0.210, 21–47, 0.030–0.105, 17–38 and 32–88 mg/kg, respectively). K2O/Al2O3, SiO2/Al2O3, and the weathering leaching coefficient (ba) showed little difference, suggesting that the weathering degree of soil in these two areas was similar. The weathering degree of soil governs the geochemical behavior of heavy metals and reference elements. According to the prediction models for heavy metal concentrations and organic carbon, K2O/Al2O3, and SiO2/Al2O3 in the soil profiles from the background area, the increase in heavy metal concentrations in the topsoil in the contaminated area was depicted. The heavy metal concentrations in topsoil were obviously affected by anthropogenic activities. This study provides a case study for evaluating the impact of anthropogenic activities on heavy metals in soil.
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来源期刊
Environmental Pollutants and Bioavailability
Environmental Pollutants and Bioavailability Chemical Engineering-Chemical Health and Safety
CiteScore
4.30
自引率
3.00%
发文量
47
审稿时长
13 weeks
期刊介绍: Environmental Pollutants & Bioavailability is a peer-reviewed open access forum for insights on the chemical aspects of pollutants in the environment and biota, and their impacts on the uptake of the substances by living organisms. Topics include the occurrence, distribution, transport, transformation, transfer, fate, and effects of environmental pollutants, as well as their impact on living organisms. Substances of interests include heavy metals, persistent organic pollutants, and emerging contaminants, such as engineered nanomaterials, as well as pharmaceuticals and personal-care products as pollutants.
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