{"title":"沼气共流扩散火焰结构、稳定性及熵产的数值分析","authors":"","doi":"10.24425/ame.2021.139648","DOIUrl":null,"url":null,"abstract":"Biogas is a gaseous biofuel predominantly composed of methane and carbon-dioxide. Stability of biogas flames strongly depend upon the amount of carbon-dioxide present in biogas, which varies with the source of biomass and reactor. In this paper, a comprehensive study on the stability and flame characteristics of coflow biogas diffusion flames is reported. Numerical simulations are carried out using reactive flow module in OpenFOAM, incorporated with variable thermophysical properties, Fick’s and Soret diffusion, and short chemical kinetics mechanism. Effects of carbon-dioxide content in the biogas, temperatures of the fuel or coflowing air streams (preheated reactant) and hydrogen addition to fuel or air streams are analyzed. Entropy generation in these flames is also predicted. Results show that the flame temperature increases with the degree of preheat of reactants and the flames show better stability with the preheated air stream. Preheating the air contributes to increased flame stability and also to a significant decrease in entropy generation. Hydrogen addition, contributing to the same power rating, is seen to be relatively more effective in increasing the flame stability when added to the fuel stream. Results in terms of flow, temperature, species and entropy fields, are used to describe the stability and flame characteristics.","PeriodicalId":1,"journal":{"name":"Accounts of Chemical Research","volume":null,"pages":null},"PeriodicalIF":16.4000,"publicationDate":"2023-11-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Numerical analysis of structure, stability and entropy generation in biogas coflow diffusion flames\",\"authors\":\"\",\"doi\":\"10.24425/ame.2021.139648\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Biogas is a gaseous biofuel predominantly composed of methane and carbon-dioxide. Stability of biogas flames strongly depend upon the amount of carbon-dioxide present in biogas, which varies with the source of biomass and reactor. In this paper, a comprehensive study on the stability and flame characteristics of coflow biogas diffusion flames is reported. Numerical simulations are carried out using reactive flow module in OpenFOAM, incorporated with variable thermophysical properties, Fick’s and Soret diffusion, and short chemical kinetics mechanism. Effects of carbon-dioxide content in the biogas, temperatures of the fuel or coflowing air streams (preheated reactant) and hydrogen addition to fuel or air streams are analyzed. Entropy generation in these flames is also predicted. Results show that the flame temperature increases with the degree of preheat of reactants and the flames show better stability with the preheated air stream. Preheating the air contributes to increased flame stability and also to a significant decrease in entropy generation. Hydrogen addition, contributing to the same power rating, is seen to be relatively more effective in increasing the flame stability when added to the fuel stream. Results in terms of flow, temperature, species and entropy fields, are used to describe the stability and flame characteristics.\",\"PeriodicalId\":1,\"journal\":{\"name\":\"Accounts of Chemical Research\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":16.4000,\"publicationDate\":\"2023-11-06\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Accounts of Chemical Research\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://doi.org/10.24425/ame.2021.139648\",\"RegionNum\":1,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Accounts of Chemical Research","FirstCategoryId":"1085","ListUrlMain":"https://doi.org/10.24425/ame.2021.139648","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
Numerical analysis of structure, stability and entropy generation in biogas coflow diffusion flames
Biogas is a gaseous biofuel predominantly composed of methane and carbon-dioxide. Stability of biogas flames strongly depend upon the amount of carbon-dioxide present in biogas, which varies with the source of biomass and reactor. In this paper, a comprehensive study on the stability and flame characteristics of coflow biogas diffusion flames is reported. Numerical simulations are carried out using reactive flow module in OpenFOAM, incorporated with variable thermophysical properties, Fick’s and Soret diffusion, and short chemical kinetics mechanism. Effects of carbon-dioxide content in the biogas, temperatures of the fuel or coflowing air streams (preheated reactant) and hydrogen addition to fuel or air streams are analyzed. Entropy generation in these flames is also predicted. Results show that the flame temperature increases with the degree of preheat of reactants and the flames show better stability with the preheated air stream. Preheating the air contributes to increased flame stability and also to a significant decrease in entropy generation. Hydrogen addition, contributing to the same power rating, is seen to be relatively more effective in increasing the flame stability when added to the fuel stream. Results in terms of flow, temperature, species and entropy fields, are used to describe the stability and flame characteristics.
期刊介绍:
Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance.
Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.