Meera Ramaswamy, Itay Griniasty, Danilo B. Liarte, Abhishek Shetty, Eleni Katifori, Emanuela Del Gado, James P. Sethna, Bulbul Chakraborty, Itai Cohen
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Nearly, all dense suspensions undergo dramatic and abrupt thickening transitions in their flow behavior when sheared at high stresses. Such transitions occur when the dominant interactions between the suspended particles shift from hydrodynamic to frictional. Here, we interpret abrupt shear thickening as a precursor to a rigidity transition and give a complete theory of the viscosity in terms of a universal crossover scaling function from the frictionless jamming point to a rigidity transition associated with friction, anisotropy, and shear. Strikingly, we find experimentally that for two different systems—cornstarch in glycerol and silica spheres in glycerol—the viscosity can be collapsed onto a single universal curve over a wide range of stresses and volume fractions. The collapse reveals two separate scaling regimes due to a crossover between frictionless isotropic jamming and frictional shear jamming, with different critical exponents. The material-specific behavior due to the microscale particle interactions is incorporated into a scaling variable governing the proximity to shear jamming, that depends on both stress and volume fraction. This reformulation opens the door to importing the vast theoretical machinery developed to understand equilibrium critical phenomena to elucidate fundamental physical aspects of the shear thickening transition.
期刊介绍:
The Journal of Rheology, formerly the Transactions of The Society of Rheology, is published six times per year by The Society of Rheology, a member society of the American Institute of Physics, through AIP Publishing. It provides in-depth interdisciplinary coverage of theoretical and experimental issues drawn from industry and academia. The Journal of Rheology is published for professionals and students in chemistry, physics, engineering, material science, and mathematics.