Ya Gao, Zezhong Xu, Yuhui Hu, Chengliang Han, Lingyun Zhang
{"title":"ag31po4 / mos2复合光催化剂的制备及其光催化性能","authors":"Ya Gao, Zezhong Xu, Yuhui Hu, Chengliang Han, Lingyun Zhang","doi":"10.1142/s0218625x24500112","DOIUrl":null,"url":null,"abstract":"Ag 3 PO 4 and MoS 2 semiconductor materials were synthesized by hydrothermal method. The composite materials were characterized by X-ray diffraction (XRD), scanning electron microscopy (SEM), X-ray energy dispersive spectroscopy (EDS), and UV–vis diffuse reflectance spectroscopy (UV–VIS DRS), and the photocatalytic degradation of organic dyes by rhodamine B was studied. The results showed that: Ag 3 PO 4 /MoS 2 composite photocatalyst is formed by using MoS 2 microspheres as the matrix and Ag 3 PO 4 nanoparticles coated on its surface or embedded in its lamellar structure. When the molar fraction of Ag 3 PO 4 in the composite product is 75%, the composite photocatalyst has better light absorption capacity and lower photogenerated carrier recombination rate (optical band gap is 1.24 eV), and shows better visible light photocatalytic degradation activity in the photocatalytic degradation of RhB experiment, the catalytic degradation rate is as high as 95.0%. At the same time, the degradation mechanism showed that H[Formula: see text] and O [Formula: see text] were the main active substances for RhB degradation. The photocatalyst has excellent performance and simple preparation method. It has broad application prospects in the field of photocatalysis.","PeriodicalId":22011,"journal":{"name":"Surface Review and Letters","volume":"52 1","pages":"0"},"PeriodicalIF":1.2000,"publicationDate":"2023-09-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"PREPARATION AND PHOTOCATALYTIC PERFORMANCE OF AG<sub>3</sub>1PO<sub>4</sub>/MOS<sub>2</sub> COMPOSITE PHOTOCATALYST\",\"authors\":\"Ya Gao, Zezhong Xu, Yuhui Hu, Chengliang Han, Lingyun Zhang\",\"doi\":\"10.1142/s0218625x24500112\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Ag 3 PO 4 and MoS 2 semiconductor materials were synthesized by hydrothermal method. The composite materials were characterized by X-ray diffraction (XRD), scanning electron microscopy (SEM), X-ray energy dispersive spectroscopy (EDS), and UV–vis diffuse reflectance spectroscopy (UV–VIS DRS), and the photocatalytic degradation of organic dyes by rhodamine B was studied. The results showed that: Ag 3 PO 4 /MoS 2 composite photocatalyst is formed by using MoS 2 microspheres as the matrix and Ag 3 PO 4 nanoparticles coated on its surface or embedded in its lamellar structure. When the molar fraction of Ag 3 PO 4 in the composite product is 75%, the composite photocatalyst has better light absorption capacity and lower photogenerated carrier recombination rate (optical band gap is 1.24 eV), and shows better visible light photocatalytic degradation activity in the photocatalytic degradation of RhB experiment, the catalytic degradation rate is as high as 95.0%. At the same time, the degradation mechanism showed that H[Formula: see text] and O [Formula: see text] were the main active substances for RhB degradation. The photocatalyst has excellent performance and simple preparation method. It has broad application prospects in the field of photocatalysis.\",\"PeriodicalId\":22011,\"journal\":{\"name\":\"Surface Review and Letters\",\"volume\":\"52 1\",\"pages\":\"0\"},\"PeriodicalIF\":1.2000,\"publicationDate\":\"2023-09-04\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Surface Review and Letters\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://doi.org/10.1142/s0218625x24500112\",\"RegionNum\":4,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q4\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Surface Review and Letters","FirstCategoryId":"1085","ListUrlMain":"https://doi.org/10.1142/s0218625x24500112","RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q4","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
PREPARATION AND PHOTOCATALYTIC PERFORMANCE OF AG31PO4/MOS2 COMPOSITE PHOTOCATALYST
Ag 3 PO 4 and MoS 2 semiconductor materials were synthesized by hydrothermal method. The composite materials were characterized by X-ray diffraction (XRD), scanning electron microscopy (SEM), X-ray energy dispersive spectroscopy (EDS), and UV–vis diffuse reflectance spectroscopy (UV–VIS DRS), and the photocatalytic degradation of organic dyes by rhodamine B was studied. The results showed that: Ag 3 PO 4 /MoS 2 composite photocatalyst is formed by using MoS 2 microspheres as the matrix and Ag 3 PO 4 nanoparticles coated on its surface or embedded in its lamellar structure. When the molar fraction of Ag 3 PO 4 in the composite product is 75%, the composite photocatalyst has better light absorption capacity and lower photogenerated carrier recombination rate (optical band gap is 1.24 eV), and shows better visible light photocatalytic degradation activity in the photocatalytic degradation of RhB experiment, the catalytic degradation rate is as high as 95.0%. At the same time, the degradation mechanism showed that H[Formula: see text] and O [Formula: see text] were the main active substances for RhB degradation. The photocatalyst has excellent performance and simple preparation method. It has broad application prospects in the field of photocatalysis.
期刊介绍:
This international journal is devoted to the elucidation of properties and processes that occur at the boundaries of materials. The scope of the journal covers a broad range of topics in experimental and theoretical studies of surfaces and interfaces. Both the physical and chemical properties are covered. The journal also places emphasis on emerging areas of cross-disciplinary research where new phenomena occur due to the presence of a surface or an interface. Representative areas include surface and interface structures; their electronic, magnetic and optical properties; dynamics and energetics; chemical reactions at surfaces; phase transitions, reconstruction, roughening and melting; defects, nucleation and growth; and new surface and interface characterization techniques.