用等离子体纳米粒子装饰的二氧化硅纳米线森林

A. Colombelli, M. G. Manera, R. Rella, A. Convertino
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摘要

在这项工作中,我们提出了一种新的和更便宜的等离子体材料的理论和实验分析,其潜在的生物传感应用非常有吸引力。我们研究了用球形金纳米粒子装饰的高度无序二氧化硅纳米线系统的光学性质和传感能力。由于透明二氧化硅纳米线的高扩散性,以及沿纳米线沉积的金纳米粒子所提供的选择性吸收共振,这些系统呈现出独特的光捕获特性。在LSPR共振处增强的吸收使我们的材料成为构建等离子体生物传感器的优秀候选者。通过适当的二维有限元模拟,对这些系统的光学特性进行了理论研究。作为概念的证明,我们已经成功地测试了NP/NW森林作为折射率传感器和检测蛋白质BSA - AntiBSA结合的生物分子结合的能力。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Light trapping systems for biosensor application Forest of silica nanowires decorated with plasmonic nanoparticles
In this work we present a theoretical and experimental analysis of a new and cheaper plasmonic material, very attractive for its potential biosensing applications. We investigate the optical properties and the sensing capabilities of a highly disordered system of silica nanowires decorated with spherical gold nanoparticles. These systems present unique light trapping properties due to the combination of the highly diffusivity of transparent silica nanowires, with the selective absorption resonances given by Au nanoparticles deposited along the wires. The enhanced absorption at the LSPR resonances makes our materials excellent candidates to build plasmonic biosensors. The optical properties of these systems have been theoretically investigated by developing appropriate 2D finite element simulations. As proof of concept we have successfully tested the ability of the NP/NW forests to act as refractive index sensors and to detect biomolecular binding of the Protein BSA - AntiBSA bonding.
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