{"title":"时间分辨受激拉曼实验","authors":"M. V. Exter, A. Lagendijk","doi":"10.1063/1.35765","DOIUrl":null,"url":null,"abstract":"We have performed time‐resolved stimulated Raman experiments on CS2, benzene and diamond. These time‐resolved SRS measurements produce more information than ordinary Raman or even non‐time‐resolved (two beams) SRS experiments because the signal is sensitive to the optical phases of the laser beams and registers therefore the so‐called electronic contribution.Finally we discuss the (im)possibility to resolve an inhomogeneously broadened line in its homogeneous components using the time‐resolved Raman technique. Computer simulations support our theoretical analysis.","PeriodicalId":298672,"journal":{"name":"Advances in Laser Science-I","volume":"183 1","pages":"0"},"PeriodicalIF":0.0000,"publicationDate":"2008-06-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Time‐resolved stimulated Raman experiments\",\"authors\":\"M. V. Exter, A. Lagendijk\",\"doi\":\"10.1063/1.35765\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"We have performed time‐resolved stimulated Raman experiments on CS2, benzene and diamond. These time‐resolved SRS measurements produce more information than ordinary Raman or even non‐time‐resolved (two beams) SRS experiments because the signal is sensitive to the optical phases of the laser beams and registers therefore the so‐called electronic contribution.Finally we discuss the (im)possibility to resolve an inhomogeneously broadened line in its homogeneous components using the time‐resolved Raman technique. Computer simulations support our theoretical analysis.\",\"PeriodicalId\":298672,\"journal\":{\"name\":\"Advances in Laser Science-I\",\"volume\":\"183 1\",\"pages\":\"0\"},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2008-06-05\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Advances in Laser Science-I\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://doi.org/10.1063/1.35765\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"\",\"JCRName\":\"\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Advances in Laser Science-I","FirstCategoryId":"1085","ListUrlMain":"https://doi.org/10.1063/1.35765","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
We have performed time‐resolved stimulated Raman experiments on CS2, benzene and diamond. These time‐resolved SRS measurements produce more information than ordinary Raman or even non‐time‐resolved (two beams) SRS experiments because the signal is sensitive to the optical phases of the laser beams and registers therefore the so‐called electronic contribution.Finally we discuss the (im)possibility to resolve an inhomogeneously broadened line in its homogeneous components using the time‐resolved Raman technique. Computer simulations support our theoretical analysis.
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