松弛器的反馈模型

A. Leschhorn, H. Kliem
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引用次数: 2

摘要

我们建立了一个模型来模拟弛豫器的行为,例如它们在宽温度范围内的高介电常数。我们的模型是基于在本质不对称双阱势中热激活的波动电荷。这种不对称是由无序引起的,可以通过局部场来调制。跃迁概率取决于势垒高度、双阱势的不对称性和局域电场。我们使用一个平均局域场,它是外加场和一个与电荷之间静电相互作用引起的极化成正比的场的叠加。这样我们就得到了极化的反馈回路。计算了具有本征不对称的双阱势中相互作用电荷系统的动态介电常数。固有的不对称性导致了弛豫行为:作为温度函数的介电常数有一个宽而高的峰值。随着频率的增加,介电常数的最大值减小并向更高的温度移动。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
A feedback model for relaxors
We develop a model to simulate the behavior of relaxors, e.g. their high permittivity in a broad temperature range. Our model is based on charges fluctuating thermally activated in intrinsically asymmetric double well potentials. The asymmetry is caused by disorder and can be modulated by a local field. The transition probabilities depend on the barrier height, the asymmetries of the double well potentials and on the local electric field. We use a mean local field which is the superposition of the applied field and a field proportional to the polarization due to the electrostatic interaction between the charges. In that way we get a feedback loop for the polarization. The dynamic permittivity is computed for systems of interacting charges in double well potentials with intrinsic asymmetry. The intrinsic asymmetry causes relaxor behavior: the permittivity as function of the temperature has a broad and high peak. The maximum of the permittivity decreases and is shifted to higher temperatures with increasing frequency.
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