等离子体与二维材料:平面上增强的光-物质相互作用(会议报告)

Koray Aydin
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引用次数: 0

摘要

单层二维过渡金属二硫族化合物(2D-TMDCs)因其理想的输运性质和直接带隙而受到广泛关注,并在现代纳米电子和光电子应用方面进行了大量研究。已知这些特性只发生在TMDCs中,当被稀释成一个或几个单层时。然而,由于半导体材料的体积决定了较差的光吸收和发射,因此降维对光子学和光电子学应用提出了重大挑战。等离子体纳米结构被广泛研究用于增强各种材料系统中的光-物质相互作用,从而增加发射和吸收性能。二维材料提供了材料厚度的最终下限,因此,以增强光-物质相互作用为特定目标的等离子体/二维材料混合材料系统的研究对于实际光电应用至关重要。在这次演讲中,我将讨论使用周期性等离子体纳米圆盘阵列和单个等离子体光学天线来增加MoS2的光致发光发射。我还将描述一种方法,用于理解和识别使用锥形金天线的激发和发射场增强对整体光致发光增强的贡献。此外,我将描述一个系统的研究,其中我们已经证明单层WS2薄膜增加了光吸收。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Plasmonics meet 2D materials: enhanced light-matter interactions in the flatland (Conference Presentation)
Monolayer two-dimensional transition metal dichalcogenides (2D-TMDCs) have gained immense attention for their desirable transport properties and direct bandgap that have led to a plethora of studies on modern nanoelectronic and optoelectronic applications. These properties are known to occur exclusively in TMDCs when thinned down to one or few monolayers. However reduced dimensionality poses a significant challenge for photonics and optoelectronics applications due to poor light absorption and emission dictated by the volume of semiconductor material. Plasmonic nanostructures have been widely studied for enhancing light-matter interactions in wide variety of material systems resulting in increased emission and absorption properties. 2D Materials provide the ultimate lower limit in terms of material thickness, therefore investigation of plasmon/2D Material hybrid material systems with a specific aim to enhance light-matter interactions is essential for practical optoelectronic applications. In this talk, I will discuss increased photoluminescence emission from MoS2 using both periodic plasmonic nanodisc arrays as well as a single plasmonic optical antenna. I will also describe a method for understanding and identifying the contributions of excitation and emission field enhancements to the overall photoluminescence enhancement using a tapered gold antenna. Additionally, I will describe a systematic study in which we have demonstrated increased light absorption in a monolayer WS2 film.
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