F. Mei, S. Spielman, S. Hering, Jian Wang, M. Pekour, Gregory S. Lewis, B. Schmid, J. Tomlinson, Maynard Havlicek
{"title":"用于大气机载研究的多功能冷凝水粒子计数器的模拟辅助表征","authors":"F. Mei, S. Spielman, S. Hering, Jian Wang, M. Pekour, Gregory S. Lewis, B. Schmid, J. Tomlinson, Maynard Havlicek","doi":"10.5194/amt-2021-266","DOIUrl":null,"url":null,"abstract":"Abstract. Capturing the vertical profiles and horizontal variations of atmospheric aerosols often requires accurate airborne measurements. With the advantage of avoiding health and safety concerns related to the use of butanol or other chemicals, a water-based condensation particle counter (wCPC) has emerged to provide measurements under various environments. However, the airborne deployment of wCPC is relatively rare due to the lack of characterization of wCPC performance. This study investigates the performance of a commercial \"versatile\" water CPC (vWCPC Model 3789, TSI) under low-pressure conditions. The effect of conditioner temperature on wCPC performance at low pressure is examined through numerical simulation and laboratory experiments. We show that the default instrument temperature setting of 30 °C for the conditioner is not suitable for airborne measurement and that the optimal conditioner temperature for low-pressure operation is 27 °C. Additionally, we show that insufficient droplet growth becomes more significant under the low-pressure operation. The variation in the chemical composition can contribute up to 20 % uncertainty in the counting efficiency of the wCPC, but this variation is independent of pressure.\n","PeriodicalId":441110,"journal":{"name":"Atmospheric Measurement Techniques Discussions","volume":"10 1","pages":"0"},"PeriodicalIF":0.0000,"publicationDate":"2021-09-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Simulation-aided characterization of a versatile water condensation particle counter for atmospheric airborne research\",\"authors\":\"F. Mei, S. Spielman, S. Hering, Jian Wang, M. Pekour, Gregory S. Lewis, B. Schmid, J. Tomlinson, Maynard Havlicek\",\"doi\":\"10.5194/amt-2021-266\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Abstract. Capturing the vertical profiles and horizontal variations of atmospheric aerosols often requires accurate airborne measurements. With the advantage of avoiding health and safety concerns related to the use of butanol or other chemicals, a water-based condensation particle counter (wCPC) has emerged to provide measurements under various environments. However, the airborne deployment of wCPC is relatively rare due to the lack of characterization of wCPC performance. This study investigates the performance of a commercial \\\"versatile\\\" water CPC (vWCPC Model 3789, TSI) under low-pressure conditions. The effect of conditioner temperature on wCPC performance at low pressure is examined through numerical simulation and laboratory experiments. We show that the default instrument temperature setting of 30 °C for the conditioner is not suitable for airborne measurement and that the optimal conditioner temperature for low-pressure operation is 27 °C. Additionally, we show that insufficient droplet growth becomes more significant under the low-pressure operation. The variation in the chemical composition can contribute up to 20 % uncertainty in the counting efficiency of the wCPC, but this variation is independent of pressure.\\n\",\"PeriodicalId\":441110,\"journal\":{\"name\":\"Atmospheric Measurement Techniques Discussions\",\"volume\":\"10 1\",\"pages\":\"0\"},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2021-09-10\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Atmospheric Measurement Techniques Discussions\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://doi.org/10.5194/amt-2021-266\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"\",\"JCRName\":\"\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Atmospheric Measurement Techniques Discussions","FirstCategoryId":"1085","ListUrlMain":"https://doi.org/10.5194/amt-2021-266","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
引用次数: 0
摘要
摘要捕捉大气气溶胶的垂直剖面和水平变化通常需要精确的机载测量。水基冷凝粒子计数器(wCPC)的优点是避免了与使用丁醇或其他化学品有关的健康和安全问题,可以在各种环境下进行测量。然而,由于缺乏对wCPC性能的表征,wCPC的空降部署相对较少。本研究考察了商用“多功能”水CPC (vWCPC Model 3789, TSI)在低压条件下的性能。通过数值模拟和室内实验研究了调理剂温度对低压下wCPC性能的影响。我们表明,空调的默认仪表温度设置为30°C不适合机载测量,低压运行的最佳空调温度为27°C。此外,我们还表明,在低压操作下,液滴生长不足变得更加明显。化学成分的变化可以对wCPC的计数效率造成高达20%的不确定性,但这种变化与压力无关。
Simulation-aided characterization of a versatile water condensation particle counter for atmospheric airborne research
Abstract. Capturing the vertical profiles and horizontal variations of atmospheric aerosols often requires accurate airborne measurements. With the advantage of avoiding health and safety concerns related to the use of butanol or other chemicals, a water-based condensation particle counter (wCPC) has emerged to provide measurements under various environments. However, the airborne deployment of wCPC is relatively rare due to the lack of characterization of wCPC performance. This study investigates the performance of a commercial "versatile" water CPC (vWCPC Model 3789, TSI) under low-pressure conditions. The effect of conditioner temperature on wCPC performance at low pressure is examined through numerical simulation and laboratory experiments. We show that the default instrument temperature setting of 30 °C for the conditioner is not suitable for airborne measurement and that the optimal conditioner temperature for low-pressure operation is 27 °C. Additionally, we show that insufficient droplet growth becomes more significant under the low-pressure operation. The variation in the chemical composition can contribute up to 20 % uncertainty in the counting efficiency of the wCPC, but this variation is independent of pressure.