沉积在石墨烯上的单层极化粒子的电磁特性

André Souto, R. M. Pereira, Jaime E. Santos, N. Peres, M. Vasilevskiy
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摘要

有趣的等离子体效应可以从小的极化粒子与石墨烯的结合中产生,与表面等离子体极化子(SPPs)有关,后者在太赫兹(THz)光谱范围内支持SPPs。石墨烯spp与沉积在其上的纳米粒子偶极矩之间的电磁耦合产生了该系统单个组件中不存在的光学特性。当外部传播的电磁波撞击石墨烯粒子时,石墨烯中激发的spp的电磁反向作用使NPs的极化率重新归一化。此外,除了通常的偶极子-偶极子相互作用之外,通过每个粒子在石墨烯覆盖的界面上诱导的极化电荷,产生了间接的粒子-粒子耦合——这种间接耦合随着粒子间距离的变化而振荡。我们推导了考虑到所有这些影响的耦合偶极子方程,使我们能够计算粒子单层的有效光学导电性。G+NPs系统的独特特性之一是集体极化模式,导致石墨烯中太赫兹辐射吸收的显著增强,而在很宽的入射角范围内反射下降到几乎为零。这种谐振模式的频率可以通过静电门控改变石墨烯中的费米能量来调节,因此它可以用于电控太赫兹辐射的反射和传输
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Electromagnetic properties of a monolayer of polarisable particles deposited on graphene
Interesting plasmonic effects can arise from the combination of small polarisable particles with graphene, related to surface plasmon-polaritons (SPPs) supported by the latter in the terahertz (THz) spectral range. The electromagnetic coupling between graphene SPPs and dipole moments of nanoparticles (NPs) deposited on top of it gives rise to optical properties that aren’t present in the individual components of this system. The NPs’ polarisability is renormalized due to the electromagnetic back action of the SPPs which are excited in graphene when an external propagating electromagnetic wave impinges on the particle. Moreover, beyond the usual dipole-dipole interaction, an indirect particle-particle coupling arises via polarisation charges induced on the graphene-covered interface by each particle – this indirect coupling oscillates with the interparticle distance. We derived coupled-dipole equations taking into account all these effects, allowing us to calculate an effective optical conductivity of the particles’ monolayer. One of the G+NPs system’s unique properties is a collective polariton mode, causing a considerable enhancement of the THz radiation absorption in graphene, while the reflection drops to nearly zero for a broad range of angles of incidence. The frequency of this resonant mode can be adjusted by changing the Fermi energy in graphene via electrostatic gating and therefore it can be used for electrically controlled reflection and transmission of THz radiation
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