PEDOT:PSS-MAPbBr3量子点复合空穴传输层CsPbBr3钙钛矿发光二极管的研究

Chi-Ta Li, Sea-Fue Wang, You Wei, Haixing Chang, Qiming Zhao, Lung-Chien Chen
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引用次数: 0

摘要

本文研究了由聚(3,4-乙烯二氧噻吩):聚苯乙烯磺酸盐(PEDOT: PSS)和MAPbBr3量子点(QDs)组成的复杂空穴传输层(HTL)在铯-溴化铅钙钛矿发光二极管(CsPbBr3 PeLEDs)结构中的作用。MAPbBr3量子点采用液相晶体生长法在恒温条件下形成的MAPbBr3块状晶体作为源材料。与PEDOT:PSS-MAPbBr3 QDs配合HTL的CsPbBr3 pleds相比,PEDOT:PSS层中的MAPbBr3 QDs明显提高了注入效率,使得注入的空穴与CsPbBr3活性层中的电子快速复合,从而减少了发射。采用PEDOT:PSS-MAPbBr3 QDs复合空穴传输层制备的CsPbBr3 pled在5.5 V电压下的最佳发光性能和外量子效率分别为10810 cd/m2和0.34%。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Study of CsPbBr3 Perovskite Light-Emitting Diodes with PEDOT:PSS-MAPbBr3 QDs Complex Hole Transport Layer
This work presents the effect of a complex hole transport layer (HTL) of poly (3,4-thylenedioxythiophene): poly(styrenesulfonate) (PEDOT: PSS) and MAPbBr3 quantum dots (QDs) in cesium lead bromide perovskite light-emitting diodes (CsPbBr3 PeLEDs) structure. The MAPbBr3 QDs used MAPbBr3 bulk crystals formed by the liquid-phase crystal growth method at constant temperature as the source material. The CsPbBr3 PeLEDs with PEDOT:PSS-MAPbBr3 QDs complexe HTL exhibited the better performance, to compare the CsPbBr3 PeLEDs with PEDOT:PSS-MAPbBr3 QDs complexe HTL, owing to the MAPbBr3 QDs in PEDOT:PSS layer apparently boosted injection efficiency such that the injected holes recombine with electrons in the CsPbBr3 active layer, rapidly, and then and emissions. The best results of luminescence and external quantum efficiency of CsPbBr3 PeLEDs with PEDOT:PSS-MAPbBr3 QDs complex hole transport layer were 10810 cd/m2 and 0.34% at an applied voltage of 5.5 V, respectively.
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