金属纳米粒子附近量子点的共振荧光:量子干涉效应

Spyridon G. Kosionis, V. Yannopapas, I. Thanopulos, E. Paspalakis
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引用次数: 0

摘要

近年来,人们对半导体量子点与等离子体纳米结构耦合的量子或非线性光学特性给予了极大的关注。研究了等离子体纳米结构对量子点共振荧光光谱的影响。研究中最常见的等离子体纳米结构是金属(主要是金或银)纳米球,在大多数研究中,量子点被建模为两能级量子系统。在本工作中,我们利用量子点中自然产生的三能级v型量子系统来模拟量子点结构,并研究金属纳米球附近的共振荧光光谱。我们表明,由于金属纳米粒子的存在,特别是由于金属纳米球附近量子点的光子发射中发生的各向异性珀塞尔效应,本系统导致了量子干涉效应。然后,我们研究了量子点与金属纳米球之间不同距离的共振荧光光谱,发现共振荧光光谱从单峰光谱到多峰光谱发生了显著变化。探讨了量子干涉对共振荧光光谱的影响。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Resonance Fluorescence of a Quantum Dot near a Metallic Nanoparticle: Quantum Interference Effects
: In recent years, significant attention has been given to the quantum or nonlinear optical properties of semiconductor quantum dots coupled to plasmonic nanostructures. A phenomenon that has been studied is the modification of the resonance fluorescence spectrum of the quantum dot by the presence of the plasmonic nanostructure. The most common plasmonic nanostructure that has been studied is the metallic (mainly gold or silver) nanosphere and in most studies the quantum dot is modeled as a two-level quantum system. In this work, we model the quantum dot structure with a three-level V-type quantum system, which can naturally arise in quantum dots, and study the resonance fluorescence spectrum near a metallic nanosphere. We show that the present system leads to quantum interference effects due to the presence of the metallic nanoparticle and specifically due to the anisotropic Purcell effect that occurs in the photon emission of the quantum dot near the metallic nanosphere. We then study the resonance fluorescence spectrum, for different distances between the quantum dot and the metallic nanosphere and show that the resonance fluorescence spectrum changes significantly from a single-peak spectrum to a multipeak spectrum. The effects of quantum interference in the resonance fluorescence spectrum are also explored.
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