窄间隙强电离介质阻挡放电特性及其应用

Xiuyuan Lu, Xingquan Wang, Yuxiang Wang
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摘要

一般情况下,等离子体反应器的放电间隙大于1mm,导致气体电离程度较弱,氧活性粒子较少。为了提高等离子体反应器中电离气体的强度,获得高浓度的氧活性粒子,采用石英作为阻挡介质,设计了放电间隙小于0.3 mm的同轴等离子体反应器。本文研究了窄间隙强电离介质阻挡放电的特性及其应用。以放电O3产生量为评价指标,研究了不同电压和气体类型对等离子体反应器放电的影响。此外,还讨论了不同排放功率和曝气石对亚甲基蓝废水降解的影响。结果表明,窄间隙等离子体反应器可以实现稳定的强电离放电,放电电场强度为33.5 kV/mm。窄间隙等离子体反应器产生高浓度氧活性粒子的最佳放电电压(峰间电压)为14.2 kV。电离空气产生的O3浓度在500ppm以上,电离O2产生的O3浓度在2300ppm以上。对亚甲基蓝进行脱色的最佳放电功率为19.6 W。在曝气条件下,处理时间为3 min,亚甲蓝的脱色率可达99.48%,浓度由初始的50 mg/L降至0.26 mg/L。窄间隙等离子体反应器可以大大提高放电电场强度和放电性能。有望为工业上有机废水高效、绿色降解技术的发展提供新的思路。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Characteristics of Narrow Gap Strong Ionization Dielectric Barrier Discharge and Its Application
In general, the discharge gap of plasma reactor is larger than 1 mm, which leads to weak ionization degree of gas and less oxygen active particles. For the purpose of improving the intensity of ionized gas in plasma reactor and obtain high concentration of oxygen active particles, a coaxial plasma reactor with discharge gap less than 0.3 mm is designed by using quartz as the barrier dielectric. The characteristics of narrow gap strong ionization dielectric barrier discharge and its application are researched in this paper. Taking the amount of O3 produced by discharge as the evaluation index, the effects of different voltage and gas types on the discharge of plasma reactor have been studied. Furthermore, the effects of different discharge power and aerated stone on the degradation of methylene blue wastewater are discussed. The results show that the narrow gap plasma reactor can achieve stable strong ionization discharge and the discharge electric field strength is 33.5 kV/mm. The optimal discharge voltage (peak-to-peak voltage) is 14.2 kV for producing high concentration oxygen active particles by narrow gap plasma reactor. The concentration of O3 produced by ionizing air is above 500 ppm, the concentration of O3 produced by ionizing O2 is above 2300 ppm. Moreover, the optimal discharge power is 19.6 W for decolorization of methylene blue. Under aeration condition and treatment time for 3 min, the decolorization ratio of methylene blue can reach 99.48 %, its concentration is degraded from initial 50 mg/L to 0.26 mg/L. The narrow gap plasma reactor can greatly improve the discharge electric field strength and discharge performance. It is expected to provide a new idea for the development of efficient and green degradation technology of organic wastewater in industry.
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