The Crystal Computer - Computing with Inorganic Cellular Frameworks and Nets

The enormous potential of parallel computing has led to the first prototype devices being constructed. However, all the examples to date rely on complicated chemical and/or physical manipulations, and hence do not lend themselves to the kind of widespread investigation necessary to advance the field. This article presents a new paradigm for parallel computing: the use of solid, single crystalline materials as cellular automata suggesting the idea of the “Crystal Computer,” now possible due to a new class of crystalline cellular materials that undergo single-crystal-to-single-crystal (SC-SC) oxidation and reduction (REDOX) reactions. Two avenues are proposed for investigation: reversible single-crystal to single-crystal electronic transformations and solid-state spin transfer within spin-crossover complexes. Both schemes allow computation to occur in three dimensions, within cheap and easy to assemble materials and using commonplace techniques for input and readout.