验证中子活化计算的MCNP仿真谱与真实谱的比较

A. Markopoulos, D. Mavrikis, E. Ntalla, A. Ioannidou, A. Savidou
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引用次数: 0

摘要

退役计划的目标是获得有关装置的放射学知识。这一阶段的表征可以通过以下方法进行:(a)基于反应堆设计和中子通量的中子活化计算;(b)剂量率测量;(c)原位伽马能谱法;(d)取样以确定活化和污染组分中的比例因子。中子活化计算包含几个不确定因素。这些不确定性基于输入数据——例如材料数据(成分和杂质)、中子通量和能量、核数据库——以及过程的方法和模拟代码。考虑到所有这些建模的不确定性,本工作的重点是开发一种验证计算的技术。目前正在开发一种利用MCNP6模拟的非破坏性伽马能谱技术,用于解释活性组分中放射性核素的伽马能谱。特别是,将根据活化组分中主要放射性核素的活性和MCNP6模拟的结果产生一个光谱。该光谱将与实验光谱进行比较。此外,在退役决策过程中,活性组分的放射学表征对表面污染至关重要。为减少二次废物的产生和限制对人员的剂量而采用的切割技术和选择除污技术应以准确确定材料内部和/或表面污染中的放射性核素为基础。所提出的方法在这种情况下也可能有所帮助。利用比例因子和剂量率测量产生的活性,将实验谱与MCNP6模拟产生的活性进行比较,可以确定组分内部和表面的活性。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Comparison of Real and Generated by MCNP Simulation Spectrums for Validation of Neutron Activation Calculations
The objective for decommissioning planning, is to obtain a radiological understanding of the involved installation. The characterization at this stage could be carried out by means of: (a) neutron activation calculations based on reactor design and neutron flux; (b) dose rate measurements; (c) in-situ gamma spectrometry; (d) sampling for determination of the scaling factors in activated and contaminated components.Neutron activation calculations contains several uncertainties. These uncertainties are based on the input data - such as material data (composition and impurities), neutron flux and energy, nuclear data libraries - and on the methodology of the process and the simulation codes.Taking into consideration all these modeling uncertainties, this work is focused on the development of a technique for validation of the calculations. A non-destructive gamma spectrometry technique by using MCNP6 simulations is under development for interpretation of the resulting gamma-ray spectra of the radionuclides in activated components. In particular, a spectrum will be produced, based on the activities of the main radionuclides in the activated component and the results of MCNP6 simulations. This spectrum will be compared with the experimental spectrum.Furthermore, the radiological characterization of activated components, which appeared with surface contamination, is essential for the decision making process during decommissioning. The cutting techniques to be followed in order to reduce the production of secondary waste and limit the doses to personnel and the selection of decontamination techniques should be based on accurate determination of the radionuclides inside the material and/ or in the surface contamination. The proposed method could also be helpful in this case. The activities inside and on the surface of the components could be determined by comparing the experimental spectrum with that produced by MCNP6 simulations, using the arisen activities from the scaling factors and the dose rate measurements.
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