OPSE、SHRS、FWPM的非线性光学过程及其竞争

Feng Zhang, Yu‐yang Zhang, T. Sun
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引用次数: 0

摘要

对Na 3S-4D双光子共振激发引起的复杂非线性光学过程进行了深入研究,并对其在2.34μm附近产生的相干辐射进行了测量和分析。通过对前向和后向输出的观察,认为该复杂过程由光泵浦受激发射(OPSE)、受激超拉曼散射(SHRS)和四波参量混频(FWPM)组成。它们往往同时并存,在不同的条件下,相互支配,相互之间存在着明显的竞争。通过调节实验条件,如介质温度、输入光频率和相互作用长度,可以获得较高的转换效率。在此工作中产生的以2.34μm为中心的相干1R辐射在300cm-1范围内可调谐,峰值功率为100 kW,效率为2%。首次观测到18条新的相干紫外线
本文章由计算机程序翻译,如有差异,请以英文原文为准。
The Nonlinear Optical Processes of OPSE,SHRS,FWPM and Their Competitions
The complex nonlinear optical process induced by two-photon-resonant excitation of Na 3S-4D has been thoroughly studied and the generated coherent radiation in the vicinity of 2.34μm measured and analysed.Based on the observation of forward and backward output it is believed that the complex process is composed of the optical-pumped stimulated emission (OPSE),stimulated hyper-Raman scattering (SHRS) and four-wave parametric mixing (FWPM).They often coexist simultaneously,each dominating over the others under different conditions,and there are obvious competitions among them.By adjusting experimental conditions,such as the temperature of medium,frequency of input light and interaction length,high conversion efficiency has been achieved.In this work the generated coherent 1R radiation centered at 2.34μm was tunable in 300cm-1,with a peak Dower of 100 kW,and an efficiency of 2%.18 new coherent UV lines were observed for the first time
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