水蒸汽泡微秒放电中激光诱导荧光绝对氢氧根密度和气体温度的测量

Jianan Wang, M. S. Simeni, P. Bruggeman
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引用次数: 0

摘要

尽管能够探测气相放电的激光诊断方法很多,但迄今为止,液体中气泡内发生的放电主要是通过成像和被动光学发射光谱来研究的。本文报道了用激光诱导荧光(LIF)对盐水中气泡放电的研究。在等离子体填充的气泡中测量了时间分辨绝对OH密度和气体温度。在电导率为50 mS/cm的nacl水溶液中,对针电极施加微秒电压脉冲,产生可重复性放电。针位于两个石英载玻片之间,间距为2mm。由于蒸汽泡的形成和随后的增长,在激光束的方向上达到8毫米1,气泡占据了整个间隙,并沿着石英窗的内壁膨胀。在气泡膨胀过程中,约282 nm的紫外激光束穿过气泡,带310-320 nm窄带滤波器的ICCD相机沿光束捕获空间分辨LIF信号。在气相的相同装置上,通过瑞利散射测量获得了绝对OH liff信号的校准。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Laser-Induced Fluorescence Absolute OH Density and Gas Temperature Measurements in a Water Vapor Bubble Microsecond Discharge
Despite the extensive list of laser diagnostics capable of probing gas phase discharges, electrical discharges occurring inside bubbles in liquids have to date mainly been investigated by imaging and passive optical emission spectroscopy. In this paper, we report an investigation of a bubble discharge in liquid saline water using laser-induced fluorescence (LIF). Time-resolved absolute OH density and gas temperature are measured in the plasma-filled bubble. The reproducible discharge was generated by applying a microsecond voltage pulse to a needle electrode submerged in a NaCl-water solution with a conductivity of 50 mS/cm. The needle was located between two quartz slides with a gap distance of 2 mm. Due to the formation and subsequent growth of a vapor bubble becoming as large as 8 mm1 in the direction of the laser beam, the bubble occupies the entire gap and expands along the inner wall of quartz windows. During this bubble expansion, a UV laser beam around 282 nm was passed through the bubble and an ICCD camera with a narrowband filter (310–320 nm) was capturing the spatially resolved LIF signal along the laser beam. Absolute OH LIF signal calibration was obtained from Rayleigh scattering measurements on the same setup in gas phase.
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