大气放电等离子体中活性物质的激光光谱诊断

C. Feng, Zhiwei Wang, H. Ding
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引用次数: 0

摘要

表面微放电(SMD)是冷大气压等离子体(CAPS)的一种,由于其良好的特性,在航空航天和生物医学等领域有着广阔的应用前景。值得注意的是,反应性化学物质是关键的促成因素,并负责双重医学效应。在研究的所有CAP源中,SMD阵列配置提供了大面积放电,具有相当大的放电体积,增强了等离子体的均匀性,并提供了大气压等离子体阵列技术的替代方案。本文研究了氦在常压脉冲调制表面微放电中OH和NO自由基的输运行为。采用激光诱导荧光测量了OH和NO自由基密度分布在脉冲持续时间和脉冲间隔时间内的时间发展。结果表明,电液动力作用下离子风引起的对流增强并主导了OH自由基从表面等离子体层向距离介电表面8 mm的余辉区域的输运。有趣的是,在等离子体关闭后,电极附近的OH密度迅速下降,但下游分布区域保持不变,这表明在放电后对流的影响仍然存在。OH的传播速度随时间单调下降。在等离子体开启的前1ms内,估计其最大值为1.86 m/s。研究了输出功率对等离子体的影响,结果表明,探测区各处的氢氧密度与施加功率成正比。然而,输入功率对传播速度和传递距离没有显著影响,表明通过增加传递到等离子体的功率来增加反应物质的传递距离是不现实的。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Laser Spectroscopic Diagnosis of Active Species in Atmospheric Discharge Plasma
Surface micro-discharge (SMD), one type of cold atmospheri c pressure plasmas (CAPS), promises a bright future for num erous applications spanning the fields of aerospace and biom edicine due to its desirable features. Significantly, the reactiv e chemical species are key enablers and responsible for the bi omedical effects. Of all the CAP sources under investigation, the SMD array configuration offers a large area discharge wit h a considerable discharge volume enhances the plasma unifo rmity and provides an alternative to atmospheric pressure pla sma array technologies. This work presents the transport beh avior investigation of OH as well as NO radicals in an atmos pheric pressure pulsed-modulated surface micro-discharge in helium. Laser-induced fluorescence is employed to measure t he time development of OH and NO radical density distributi on during the pulse duration and the inter-pulse period. It is s hown that convection caused by ion wind due to electro hydr odynamic force enhances and dominates the transport of OH radicals from the surface plasma layer to the afterglow region with a distance up to 8 mm away from the dielectric surface. Interestingly, after the plasma switches off, OH density decre ases quickly near the electrode but the downstream distributi on region keeps constant, showing that the impact of convecti on is still present during the post-discharge. Additionally, the propagation velocity of OH declines monotonously with time. The maximum value is estimated as 1.86 m/s during the first 1 ms when the plasma is on. The influence of power delivere d to plasma is investigated, and the results indicate that the O H density everywhere in the detection zone is directly proport ional to the applied power. However, the input power has no significant influence on the propagation velocity and delivery distance, suggesting that it is unrealistic to increase the deliv ery distance of reactive species by increasing the power deliv ered to plasma.
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