CdSe胶体纳米晶体发射的低温相干时间测量

L. Coolen, X. Brokmann, E. Giacobino, M. Dahan, J. Hermier
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引用次数: 0

摘要

本文报道了CdSe纳米晶体荧光时间相干性的精确测量。在低温下,发射线宽预计低于0.2 meV,由于光谱仪分辨率不足和发射波长的光谱扩散,直接测量线宽是不可能的。为了获得更高的分辨率,使用了迈克尔逊干涉仪。提出了一种新颖的高灵敏度方法,该方法基于在两个干涉仪输出处检测到的光子之间的时间相关性。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Low-temperature coherence-time measurements for CdSe colloidal nanocrystals emission
In this paper, precise measurement of the time coherence of CdSe nanocrystals fluorescence is reported. At low temperature, where emission linewidth is expected to be below 0.2 meV, direct linewidth measurements are not possible, due to insufficient spectrometer resolution and spectral diffusion of the emission wavelength. To obtain a higher resolution, Michelson interferometer is used. An original highly sensitive method, based on the time-correlation between the photons detected at the two interferometer outputs is developed.
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