单壁碳纳米管中高能拉曼模式的起源

Structural and Electronic Properties of Molecular Nanostructures. XVI International Winterschool on Electronic Properties of Novel Materials Pub Date : 2002-10-02 DOI:10.1063/1.1514139

J. Maultzsch, C. Thomsen, S. Reich, M. Machoň

{"title":"单壁碳纳米管中高能拉曼模式的起源","authors":"J. Maultzsch, C. Thomsen, S. Reich, M. Machoň","doi":"10.1063/1.1514139","DOIUrl":null,"url":null,"abstract":"We present a new interpretation of the origin of the first‐order Raman modes in single‐wall carbon nanotubes. Similar to the disorder‐induced D mode, the high‐energy modes are determined by double‐resonant scattering. Our model predicts an excitation‐energy dependence of the Raman frequencies, which we observe experimentally as well. We present preliminary results on the Raman spectra of metallic tubes.","PeriodicalId":196292,"journal":{"name":"Structural and Electronic Properties of Molecular Nanostructures. XVI International Winterschool on Electronic Properties of Novel Materials","volume":"37 1","pages":"0"},"PeriodicalIF":0.0000,"publicationDate":"2002-10-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"1","resultStr":"{\"title\":\"Origin of the high‐energy Raman modes in single‐wall carbon nanotubes\",\"authors\":\"J. Maultzsch, C. Thomsen, S. Reich, M. Machoň\",\"doi\":\"10.1063/1.1514139\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"We present a new interpretation of the origin of the first‐order Raman modes in single‐wall carbon nanotubes. Similar to the disorder‐induced D mode, the high‐energy modes are determined by double‐resonant scattering. Our model predicts an excitation‐energy dependence of the Raman frequencies, which we observe experimentally as well. We present preliminary results on the Raman spectra of metallic tubes.\",\"PeriodicalId\":196292,\"journal\":{\"name\":\"Structural and Electronic Properties of Molecular Nanostructures. XVI International Winterschool on Electronic Properties of Novel Materials\",\"volume\":\"37 1\",\"pages\":\"0\"},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2002-10-02\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"1\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Structural and Electronic Properties of Molecular Nanostructures. XVI International Winterschool on Electronic Properties of Novel Materials\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://doi.org/10.1063/1.1514139\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"\",\"JCRName\":\"\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Structural and Electronic Properties of Molecular Nanostructures. XVI International Winterschool on Electronic Properties of Novel Materials","FirstCategoryId":"1085","ListUrlMain":"https://doi.org/10.1063/1.1514139","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}

引用次数: 1

摘要

我们对单壁碳纳米管中一阶拉曼模式的起源提出了新的解释。与无序诱导的D模式类似，高能量模式是由双共振散射确定的。我们的模型预测了喇曼频率的激发能依赖性，我们也通过实验观察到了这一点。本文给出了金属管拉曼光谱的初步结果。

本文章由计算机程序翻译，如有差异，请以英文原文为准。

查看原文本刊更多论文

Origin of the high‐energy Raman modes in single‐wall carbon nanotubes

We present a new interpretation of the origin of the first‐order Raman modes in single‐wall carbon nanotubes. Similar to the disorder‐induced D mode, the high‐energy modes are determined by double‐resonant scattering. Our model predicts an excitation‐energy dependence of the Raman frequencies, which we observe experimentally as well. We present preliminary results on the Raman spectra of metallic tubes.

求助全文

通过发布文献求助，成功后即可免费获取论文全文。去求助

来源期刊

Structural and Electronic Properties of Molecular Nanostructures. XVI International Winterschool on Electronic Properties of Novel Materials

自引率

0.00%

发文量