球形纳米天线周围N二能级量子系统的共振荧光光谱

ALT Proceedings Pub Date : 2012-11-01 DOI:10.12684/ALT.1.85
Y. Vladimirova, V. Klimov, V. Pastukhov, V. Zadkov
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引用次数: 0

摘要

详细研究了激光单色场对近距离等离子体纳米结构(金属球)两能级原子共振荧光光谱的影响。结果表明,可以通过改变原子与纳米球之间的距离、原子在纳米球周围的位置、纳米球半径和入射辐射的极化等四个关键参数来控制该光谱。这些参数影响了与纳米球相互作用的原子的局域场增强、跃迁频移和辐射衰减率的改变,从而导致原子的共振荧光光谱(mollow型三重态中卫星线的频移、线的宽度和光谱强度)与自由空间中的共振荧光光谱相比发生了变化。金属纳米层的介电常数也是一个附加参数,它定义了非辐射衰变。后者与其他参数相结合,可以连续控制从共振荧光增强到其猝灭的转变。计算结果推广到n个两能级原子分布在纳米粒子表面附近的情况。对探测器相对于系统纳米粒子原子的不同位置进行了计算。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
The resonance fluorescence spectra of N two-level quantum systems located around the spherical nanoantenna
Modification of the resonance fluorescence spec-trum of a two-level atom driving by a lasermonochromatic field in the close proximity of aplasmonic nanostructure (metal sphere) is studiedin detail. It is shown that one can control thisspectrum varying four key parameters: distancebetween the atom and the nanosphere, atom’s lo-cation around the nanosphere, the radius of thenanosphere, and polarization of the incident ra-diation. These parameters affect the local fieldenchancement, transition frequency shift and themodification of the radiative decay rate of the atominteracting with the nanosphere, which lead tomodification of the resonance fluorescence spec-trum of the atom (frequency shift of the satellitelines in the Mollow-type triplet, widths of the lines,the spectrum intensity) by contrast with that onein free space. The permittivity of the metal thenanosphere is made of is also an additional param-eter, which defines the nonradiative decay. The lat-ter in combination with other parameters allows tocontinuously control the transition from resonancefluorescence enhancement to its quenching. Thecalculation results are generalized to the case ofN two-level atoms, distributed around the nanopar-ticle in the close proximity of its surface. Thecalculations were performed for different positionsof the detector relative to the system nanoparticle-atom(s).
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