2014-2019年天气环流对东南沿海生态城市地表臭氧污染的影响

IF 6.9 Q1 Environmental Science
Yu Yan , Xuesong Wang , Zhengchao Huang , Kun Qu , Wenbin Shi , Zimu Peng , Limin Zeng , Shaodong Xie , Yuanhang Zhang
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引用次数: 3

摘要

近年来,中国东南部沿海生态城市福州不时出现严重的臭氧(O3)事件。本研究采用主观方法确定了2014-2019年福州市影响80%以上O3污染天数的三种典型天气环流类型。总结了三种CT条件下与O3光化学形成和传输有关的气象条件特征。应用可扩展的综合空气质量模型对福州市不同地区的O3事件进行了模拟和量化。当福州位于高压系统(被归类为“东脊”)的西部时,更多温暖的西南气流流向福州,广东省的跨区域输送和当地高产量的影响促进了O3事件的发生。在福州以东低压系统(定义为“东低”)的均匀压力场下,停滞的天气条件导致大气边界层中O3的局地产生最强。受大陆高压系统(被归类为“内陆高压”)的控制,偏北气流增强了跨区域输送对福州O3的贡献。2018年4月和5月,“东脊”和“内陆高压”的异常增加与福州的O3污染密切相关,导致近年来O3污染日数达到年最大值。此外,2017-2019年秋季O3事件数量的增加主要与“内陆高压”有关,这表明跨区域运输的加剧,并突出了加强区域合作和努力应对O3污染的必要性。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Impacts of synoptic circulation on surface ozone pollution in a coastal eco-city in Southeastern China during 2014-2019

The coastal eco-city of Fuzhou in Southeastern China has experienced severe ozone (O3) episodes at times in recent years. In this study, three typical synoptic circulations types (CTs) that influenced more than 80% of O3 polluted days in Fuzhou during 2014-2019 were identified using a subjective approach. The characteristics of meteorological conditions linked to photochemical formation and transport of O3 under the three CTs were summarized. Comprehensive Air Quality Model with extensions was applied to simulate O3 episodes and to quantify O3 sources from different regions in Fuzhou. When Fuzhou was located to the west of a high-pressure system (classified as “East-ridge”), more warm southwesterly currents flowed to Fuzhou, and the effects of cross-regional transport from Guangdong province and high local production promoted the occurrence of O3 episodes. Under a uniform pressure field with a low-pressure system occurring to the east of Fuzhou (defined as “East-low”), stagnant weather conditions caused the strongest local production of O3 in the atmospheric boundary layer. Controlled by high-pressure systems over the mainland (categorized as “Inland-high”), northerly airflows enhanced the contribution of cross-regional transport to O3 in Fuzhou. The abnormal increases of the “East-ridge” and “Inland-high” were closely related to O3 pollution in Fuzhou in April and May 2018, resulting in the annual maximum number of O3 polluted days during recent years. Furthermore, the rising number of autumn O3 episodes in 2017-2019 was mainly related to the “Inland-high”, indicating the aggravation of cross-regional transport and highlighting the necessity of enhanced regional collaboration and efforts in combating O3 pollution.

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来源期刊
Journal of environmental sciences
Journal of environmental sciences Environmental Science (General)
CiteScore
12.80
自引率
0.00%
发文量
0
审稿时长
17 days
期刊介绍: Journal of Environmental Sciences is an international peer-reviewed journal established in 1989. It is sponsored by the Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, and it is jointly published by Elsevier and Science Press. It aims to foster interdisciplinary communication and promote understanding of significant environmental issues. The journal seeks to publish significant and novel research on the fate and behaviour of emerging contaminants, human impact on the environment, human exposure to environmental contaminants and their health effects, and environmental remediation and management. Original research articles, critical reviews, highlights, and perspectives of high quality are published both in print and online.
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