Uranium in the Arabian Sea: role of denitrification in controlling its distribution

R Rengarajan, M.M Sarin, S Krishnaswami
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引用次数: 19

Abstract

A total of 61 samples, from six vertical profiles between surface and 1800 m from the Arabian Sea, have been analysed for uranium concentration to assess its behaviour in oxic and sub-oxic waters. These samples cover a wide range of dissolved oxygen concentration, from 0.14 to 230 μM. Uranium concentration in most of the samples fall in the range of 3.2 ± 0.2 μg l–1. In general, uranium exhibits a conservative behaviour in the Arabian Sea water column and denitrification processes do not seem to influence its abundance. The mean uranium/salinity ratio in waters with dissolved oxygen <2 μM is (9.17 ± 0.15) × 10–8 g g–1, nearly identical to the ratio (9.22 ± 0.27) × 10–8 g g–1 in waters with dissolved oxygen >100 μM, and in waters from other oceanic regions (9.34 ± 0.56) × 10–8 g g–1. In one of the profiles (18°N, 64°E) collected during summer monsoon (SK115/6; August 1996), two samples from 300 and 600 m have uranium concentration ∼10–15% lower than that expected based on salinity. Further studies are needed to confirm these results and to characterize the process(es) contributing to depletion of uranium at these depths.

阿拉伯海中的铀:反硝化作用在控制其分布中的作用
从阿拉伯海表面到1800米之间的6个垂直剖面共61个样本进行了铀浓度分析,以评估其在含氧和亚含氧水域中的行为。这些样品的溶解氧浓度范围为0.14 ~ 230 μM。大部分样品的铀浓度在3.2±0.2 μg - 1范围内。一般来说,铀在阿拉伯海水柱中表现出保守的行为,反硝化过程似乎不影响其丰度。2 μM溶解氧水体的平均铀盐比为(9.17±0.15)× 10-8 g - 1,与100 μM溶解氧水体的平均铀盐比为(9.22±0.27)× 10-8 g - 1和其他海域的平均铀盐比为(9.34±0.56)× 10-8 g - 1基本一致。在夏季风期间收集的一条剖面(18°N, 64°E) (SK115/6;1996年8月),来自300和600米的两个样品的铀浓度比根据盐度预期的低~ 10-15%。需要进一步的研究来证实这些结果,并描述导致这些深度的铀枯竭的过程。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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