Radioisotope Identification with Scintillation Detector Based on Artificial Neural Networks Using Simulated Training Data

Peng Fan, Siliang Feng, Chenglin Zhu, Chunqing Zhao, Y. Ding, Zicai Shen, Yaqiang Liu, Tianyu Ma, Y. Xia
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Abstract

Artificial neural networks (ANN) based on learning the features of the entire measured gamma energy spectrum has been used for radioisotope identification and proved promising especially for gamma-ray spectroscopy with low energy resolution. The implementation of ANN method, however, requires tedious experimental measurement process in generation of training data for various radioisotopes. In this work, we propose an ANN-based radioisotope identification method with simulated training data. Gamma energy spectra of 27 different radioisotopes were generated with Monte Carlo simulation. A detector energy response model was proposed to match the energy spectra generated from simulation and measured from experiment, thus “pseudo” measured energy spectra of various radioisotopes transformed from simulation can be used for ANN training, which eliminates the tedious experimental measurement process for training data generation. To reduce the complexity of the training process, the principal component analysis (PCA) method was used for dimension reduction of the input energy spectra in ANN and the channel number of the energy spectra was reduced from 2000 to 50. The trained ANN was further used to identify experimentally measured gamma energy spectra of various radioisotopes including 60Co., 137CS., 18F, 131I, 226Ra and 232Th at 103, 104 and 105 count levels. In single isotope identification test, with increased count level, higher correct identification rate is achieved and at 105 count level, all the isotopes are correctly identified for all the samples. In mixed isotope identification test, at 105 count level, all the radioisotope combinations can be identified with a correct identification rate larger than 98%, which demonstrates the feasibility and accuracy of the ANN method. To conclude, the proposed ANN method with simulated training data features good radioisotope identification capability with greatly simplified training data generation process and is feasible for gamma spectroscopy with relatively poor energy resolution.
基于模拟训练数据的人工神经网络闪烁探测器放射性同位素识别
基于学习整个测量伽马能谱特征的人工神经网络(ANN)已被用于放射性同位素识别,特别是在低能量分辨率的伽马射线能谱中被证明是有前途的。然而,人工神经网络方法的实施需要繁琐的实验测量过程来生成各种放射性同位素的训练数据。在这项工作中,我们提出了一种基于人工神经网络的模拟训练数据的放射性同位素识别方法。用蒙特卡罗模拟生成了27种不同放射性同位素的γ能谱。提出了一种探测器能量响应模型,将模拟生成的能谱与实验测量的能谱进行匹配,从而将模拟生成的各种放射性同位素的“伪”测量能谱用于人工神经网络训练,从而消除了训练数据生成过程中繁琐的实验测量过程。为了降低训练过程的复杂性,采用主成分分析(PCA)方法对神经网络输入的能谱进行降维,并将能谱的通道数从2000个降为50个。训练后的人工神经网络进一步用于识别包括60Co在内的各种放射性同位素的实验测量γ能谱。137 cs。, 18F, 131I, 226Ra和232Th计数水平为103,104和105。在单同位素鉴定试验中,随着计数水平的增加,正确率更高,在105计数水平下,所有样品的所有同位素都被正确鉴定。在混合同位素鉴定试验中,在105个计数水平下,所有放射性同位素组合的正确率均大于98%,证明了人工神经网络方法的可行性和准确性。综上所述,基于模拟训练数据的人工神经网络方法具有良好的放射性同位素识别能力,大大简化了训练数据生成过程,对于能量分辨率相对较差的伽马能谱也是可行的。
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