M. Schwikowski, A. Döscher, H. Gäggeler, U. Schotterer
{"title":"Anthropogenic versus natural sources of atmospheric sulphate from an Alpine ice core","authors":"M. Schwikowski, A. Döscher, H. Gäggeler, U. Schotterer","doi":"10.3402/TELLUSB.V51I5.16506","DOIUrl":null,"url":null,"abstract":"Opposite to greenhouse gases, sulphate aerosol particles are expected to cause climate cooling, but uncertainties exist about source variability and strength. We analysed an ice core from a European glacier to quantify source strengths of aerosol-borne sulphate over a 200-year period. Sulphate from emissions of SO 2 increased by more than an order of magnitude during this century. This anthropogenic source is responsible for about 80% of total sulphate in the industrial period, and reflects emissions of west European countries. In the pre-industrial period mineral dust was the dominant contributor, followed by sulphate from SO 2 emissions with volcanoes or biomass burning as possible sources. DOI: 10.1034/j.1600-0889.1999.t01-4-00006.x","PeriodicalId":54432,"journal":{"name":"Tellus Series B-Chemical and Physical Meteorology","volume":null,"pages":null},"PeriodicalIF":2.3000,"publicationDate":"1999-11-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"77","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Tellus Series B-Chemical and Physical Meteorology","FirstCategoryId":"89","ListUrlMain":"https://doi.org/10.3402/TELLUSB.V51I5.16506","RegionNum":4,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"METEOROLOGY & ATMOSPHERIC SCIENCES","Score":null,"Total":0}
引用次数: 77
Abstract
Opposite to greenhouse gases, sulphate aerosol particles are expected to cause climate cooling, but uncertainties exist about source variability and strength. We analysed an ice core from a European glacier to quantify source strengths of aerosol-borne sulphate over a 200-year period. Sulphate from emissions of SO 2 increased by more than an order of magnitude during this century. This anthropogenic source is responsible for about 80% of total sulphate in the industrial period, and reflects emissions of west European countries. In the pre-industrial period mineral dust was the dominant contributor, followed by sulphate from SO 2 emissions with volcanoes or biomass burning as possible sources. DOI: 10.1034/j.1600-0889.1999.t01-4-00006.x
期刊介绍:
Tellus B: Chemical and Physical Meteorology along with its sister journal Tellus A: Dynamic Meteorology and Oceanography, are the international, peer-reviewed journals of the International Meteorological Institute in Stockholm, an independent non-for-profit body integrated into the Department of Meteorology at the Faculty of Sciences of Stockholm University, Sweden. Aiming to promote the exchange of knowledge about meteorology from across a range of scientific sub-disciplines, the two journals serve an international community of researchers, policy makers, managers, media and the general public.