Synthesis and Characterization of αFe2O4/g-C3N4 Materials for Treatment of Congo Red Dye in Water

Pham Huynh Thanh Trang, N. H. Triều, N. Trang, Nguyen Thi Hong Nham, N. M. Viet
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Abstract

In recent years, the problem of environmental pollution is becoming extremely serious. Especially, environmental pollution caused by textile dyes not only affects living organisms in the water but also affects human health. There are many methods applied to remove dyes in water; in which, photocatalysis has been proven to be an efficient method. The g-C3N4 is a polymer material with small bandgap energy (about 2,7 eV) as well as chemical and thermal stability in the ambient environment. In this study, the g-C3N4 material was successfully synthesized from urea calcined at 550 0C, and the modified materials αFe2O3/g-C3N4 were also successfully prepared by hydrothermal method. The synthesized materials were characterized by modern analytical techniques, such as SEM-EDX, XRD, UV-Vis, and FT-IR. The experimental results showed that synthesized materials have high efficiency in removing Congo Red dye in water under visible light irradiation. Especially, the 7% αFe2O3/g-C3N4 material had the best efficiency of Congo Red treatment, with an efficiency of up to 93.59% at pH 5 after 150 minutes.
αFe2O4/g-C3N4处理水中刚果红染料材料的合成与表征
近年来,环境污染问题变得极其严重。特别是纺织染料对环境的污染不仅影响水中的生物,而且影响人体健康。有许多方法用于去除水中的染料;其中,光催化已被证明是一种有效的方法。g-C3N4是一种带隙能量小(约2.7 eV)且在环境中具有化学和热稳定性的高分子材料。本研究以尿素为原料,在550℃下煅烧,成功合成了g-C3N4材料,并通过水热法制备了αFe2O3/g-C3N4改性材料。采用SEM-EDX、XRD、UV-Vis、FT-IR等现代分析技术对合成材料进行了表征。实验结果表明,在可见光照射下,合成的材料对水中刚果红染料有较好的去除效果。其中,7% αFe2O3/g-C3N4材料对刚果红的处理效率最高,在pH为5的条件下,处理时间为150 min,处理效率高达93.59%。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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