The Dependency on the Dissipation Tensor of Multi-modal Nuclear Fission

T. Asano, T. Wada, M. Ohta, S. Yamaji, H. Nakahara
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Therefore, it is supposed that the microscopic energy plays an important role for the manifestation of this phenomenon. It is a great challenge for us to understand this phenomenon in terms of nuclear many-body dynamics. Several authors studied the potential energy surface (PES) including the microscopic energy in a multi-dimensional parameter space that describes various nuclear shapes; one can deduce the possible fission paths by studying the location of the saddle points and the fission valleys in multi-dimensional parameter space. 7 With this method, they could explain the general trend of the position of the peaks of the mass distribution. The dynamical point of view is necessary to progress the study of the fission mode. We have applied the Langevin approach to the study of the fission modes in uranium nuclei and in fermium nuclei. 8–10 We studied the mass and TKE distributions and demonstrated that we can decompose the fission events into several components by tracing the Langevin trajectories. We also studied the isotope dependence and the excitation energy dependence of the fission mode. 8–10 In the previous studies, we adopted the wall-and-window type one-body friction as the dissipation mechanism of the nuclear fission dynamics. The validity of this dissipation mechanism has been demonstrated by one of the authors (T.W.) who studied the dissipation tensor dependence of the pre-scission neutron multiplicity and the mean TKE. 11–14 From the comparison of the results of the dynamical calculation with experimental data, they excluded the possibility of the two-body type dissipation to be the dominant mechanism by showing that it cannot reproduce the pre-scission neutron data and the TKE data simultaneously. On the other hand, they showed that the wall-and-window type one-body friction can reproduce both data reasonably well and concluded that it is a reasonable model for the dissipation mechanism of nuclear fission. There are other models that are of one-body nature, e.g. surface-plus-window formula, modified wall-and-window formula and chaos weighted wall formula. 15–17 Though there were no free parameters in the original derivation of the one-body friction, 18, 19 the strength has been modified frequently in order to reproduce some experimental data. For example, in the study of the light particle evaporation and the mass distribution, Schmitt et al. used the strength as a free parameter. 17 The modification itself should be acceptable when we take account of the simplicity of the model; it is a macroscopic model without any microscopic effect and it has no dependence on the temperature. However, when one modifies the strength of the nuclear dissipation just to reproduce only one physical quantity, it might be inappropriate to conclude that the deduced strength has definite physical meanings. 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引用次数: 13

Abstract

In the study of the fission of actinide nuclei at low excitation energies including the spontaneous fission, it was found that the fragment mass distribution and the total kinetic energy (TKE) distribution consist of more than one component, in contrast to the simple single peak structure that is found in the fission at high excitation energies. 1– 6 This phenomenon is attributed to the existence of more than one fission path and is called the multi-modal fission. The mass and TKE distributions depend sensitively on the excitation energy and the position of the peaks of the mass distribution suggests the influence of the closed shell structure of the fragments. Therefore, it is supposed that the microscopic energy plays an important role for the manifestation of this phenomenon. It is a great challenge for us to understand this phenomenon in terms of nuclear many-body dynamics. Several authors studied the potential energy surface (PES) including the microscopic energy in a multi-dimensional parameter space that describes various nuclear shapes; one can deduce the possible fission paths by studying the location of the saddle points and the fission valleys in multi-dimensional parameter space. 7 With this method, they could explain the general trend of the position of the peaks of the mass distribution. The dynamical point of view is necessary to progress the study of the fission mode. We have applied the Langevin approach to the study of the fission modes in uranium nuclei and in fermium nuclei. 8–10 We studied the mass and TKE distributions and demonstrated that we can decompose the fission events into several components by tracing the Langevin trajectories. We also studied the isotope dependence and the excitation energy dependence of the fission mode. 8–10 In the previous studies, we adopted the wall-and-window type one-body friction as the dissipation mechanism of the nuclear fission dynamics. The validity of this dissipation mechanism has been demonstrated by one of the authors (T.W.) who studied the dissipation tensor dependence of the pre-scission neutron multiplicity and the mean TKE. 11–14 From the comparison of the results of the dynamical calculation with experimental data, they excluded the possibility of the two-body type dissipation to be the dominant mechanism by showing that it cannot reproduce the pre-scission neutron data and the TKE data simultaneously. On the other hand, they showed that the wall-and-window type one-body friction can reproduce both data reasonably well and concluded that it is a reasonable model for the dissipation mechanism of nuclear fission. There are other models that are of one-body nature, e.g. surface-plus-window formula, modified wall-and-window formula and chaos weighted wall formula. 15–17 Though there were no free parameters in the original derivation of the one-body friction, 18, 19 the strength has been modified frequently in order to reproduce some experimental data. For example, in the study of the light particle evaporation and the mass distribution, Schmitt et al. used the strength as a free parameter. 17 The modification itself should be acceptable when we take account of the simplicity of the model; it is a macroscopic model without any microscopic effect and it has no dependence on the temperature. However, when one modifies the strength of the nuclear dissipation just to reproduce only one physical quantity, it might be inappropriate to conclude that the deduced strength has definite physical meanings. It may reflect the other effects completely different from the dissipation, like the insufficiency of the model space. It is very important to compare many (at least more than one) physical quantities at the same time. Among the physical quantities that are measured in nuclear fission, the TKE and mass distributions are well investigated experimentally in many cases. In this study, we use these quantities to discuss the dissipation dependence of the fission modes. It is shown that the TKE distribution is, as was expected, directly connected to the strength of the dissipation and we can put some constraints on the strength of the dissipation. Furthermore, it is shown that the mass distribution changes rather drastically when one uses different models for the dissipation mechanism. These results demonstrate the importance and the usefulness of the dynamical approach to the study of the fission mode. Section 2 gives a concise description of our framework. Results are shown in Sec. 3 concerning the fission of 264 Fm nucleus at Ex = 20 MeV. Summary is given in Sec. 4. 2. Methods
多模态核裂变对耗散张量的依赖
在对包括自发裂变在内的锕系原子核低激发能裂变的研究中,发现碎片质量分布和总动能(TKE)分布由多个分量组成,而不是高激发能裂变的简单单峰结构。这种现象归因于不止一个裂变路径的存在,被称为多模态裂变。碎片的质量和TKE分布敏感地依赖于激发能,质量分布峰的位置反映了碎片闭合壳结构的影响。因此,我们认为微观能量对这一现象的表现起着重要的作用。从核多体动力学的角度来理解这一现象对我们来说是一个巨大的挑战。一些作者研究了势能面(PES),包括描述各种核形状的多维参数空间中的微观能量;通过研究鞍点和裂变谷在多维参数空间中的位置,可以推断出可能的裂变路径。用这种方法,他们可以解释质量分布的峰的位置的一般趋势。动力学的观点对推进裂变模式的研究是必要的。我们已经将朗之万方法应用于铀核和镄核的裂变模式的研究。8-10我们研究了质量和TKE分布,并证明我们可以通过跟踪朗之万轨迹将裂变事件分解为几个分量。我们还研究了裂变模式的同位素依赖性和激发能依赖性。8-10在以往的研究中,我们采用墙窗式的一体摩擦作为核裂变动力学的耗散机制。这一耗散机制的有效性已被一位作者(T.W.)证明,他研究了裂变前中子多重度和平均TKE的耗散张量依赖关系。从动力学计算结果与实验数据的比较中,他们排除了二体型耗散作为主要机制的可能性,表明它不能同时再现裂变前中子数据和TKE数据。另一方面,他们证明了墙窗型一体摩擦可以很好地再现这两个数据,并得出结论,它是核裂变耗散机制的合理模型。还有一些单体模型,如曲面加窗公式、修正墙窗公式和混沌加权墙公式。虽然在最初的单体摩擦推导中没有自由参数18,19,但为了再现一些实验数据,强度经常被修改。例如,Schmitt等人在研究轻粒子蒸发和质量分布时,使用强度作为自由参数。考虑到模型的简单性,修改本身应该是可以接受的。这是一个没有任何微观影响的宏观模型,它不依赖于温度。然而,当人们修改核耗散强度只是为了再现一个物理量时,推断出的强度具有确定的物理意义可能是不恰当的。它可能反映了与耗散完全不同的其他效应,如模型空间的不足。同时比较许多(至少不止一个)物理量是非常重要的。在核裂变测量的物理量中,TKE和质量分布在许多情况下都得到了很好的实验研究。在本研究中,我们使用这些量来讨论裂变模式的耗散依赖性。结果表明,TKE分布与耗散强度直接相关,我们可以对耗散强度施加一定的约束。此外,当使用不同的耗散机制模型时,质量分布变化相当大。这些结果证明了用动力学方法研究裂变模式的重要性和实用性。第2节简要描述了我们的框架。关于264fm核在Ex = 20mev时裂变的结果见第3节。第4节给出了摘要。2. 方法
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