Study of Hydrogen Sulfide Removal Using Dielectric Barrier Discharge

H. Fang, Jian Li, W. Liang, Jing-xin Li, Y. Liu, Yuquan Jin
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Abstract

An experimental research on hydrogen sulfide removal by DBD was carried out. This study explored the influences of initial concentration ,gas flow rate, applied voltage and frequency on hydrogen sulfide removal. In addition, the differences among the no packing and ceramic raschig-ring packing in the reactor were discussed. Meanwhile, during plasma processing to decompose hydrogen sulfide, SIE was analyzed using the Q–V Lissajous diagram. The experiment data suggested that hydrogen sulfide removal efficiency raised with the addition of the applied voltage, frequency and the reducing of the initial concentration of hydrogen sulfide and gas flow; it was found that under the following conditions: applied voltage 19 kV, frequency 300 Hz, gas flow rate 8 L/min, inlet gas concentration of hydrogen sulfide 30.1 mg/m3, the hydrogen sulfide removal reached the maximum of 100%. In the presence of the packing, hydrogen sulfide removal efficiency was higher than in the case of no packing, 93.26% for the former reactor and 69.29% for the latter.
介质阻挡放电脱除硫化氢的研究
对DBD法脱除硫化氢进行了实验研究。研究了初始浓度、气体流速、施加电压和频率对硫化氢脱除的影响。此外,还讨论了反应器内无填料与陶瓷拉西格环填料的区别。同时,在等离子体处理分解硫化氢过程中,利用Q-V Lissajous图对SIE进行了分析。实验数据表明,硫化氢脱除效率随着施加电压、频率的增加、硫化氢初始浓度的降低和气体流量的减小而提高;结果表明,在施加电压19 kV、频率300 Hz、气体流速8 L/min、进口硫化氢浓度30.1 mg/m3条件下,硫化氢去除率最高可达100%。有填料时,反应器的硫化氢去除率高于无填料时,前者为93.26%,后者为69.29%。
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