Quasi-isentropic compression of LiH above 400 GPa using magnetocumulative generator.

X. Zhang, Z. Gu, Z. Xiao, F. Tan, X. Ye, Y. Tong, X. S. Tang, Z. Zhou, C. Cheng, J. Zhao, B. Luo, J. Li, X. Kuang, J. Zhao, C. W. Sun, C. L. Liu
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Abstract

The knowledge of high-pressure behavior of LiH is significant for the validation of fundamental theoretical models and applications in thermonuclear materials and potential energy supplies. The compressibility of 7LiH under isentropic compression at high pressure was investigated experimentally and theoretically. The experimental technique for quasi-isentropic compression with low-density materials was developed using the magnetocumulative generator CJ-100 and x-ray flash radiography. The x-ray images and extracted interface of the sample target in dynamic flash radiography experiments were obtained. According to each interface size of the target both before and after compression, the compression ratio of 7LiH and reference material aluminum was obtained. The density of the reference and using its known isentropic curve provide the pressure in the reference. The pressure in 7LiH was deduced from the pressure in the reference and using the calculated gradient correction factor. The quasi-isentropic data point at 438 GPa was obtained experimentally. A semiempirical three-term complete equation of state was constructed and validated for 7LiH using the theory of Mie-Grüneisen-Debye with experimental data from the literature. The quasi-isentrope data point is reasonably consistent with the theoretical results. The quasi-isentropic experimental techniques and results broaden the existing research scope and are practical and helpful to further validate theoretical models in the future.
利用磁累积发生器对400 GPa以上的LiH进行准等熵压缩。
锂离子高压行为的认识对于验证基本理论模型以及在热核材料和势能供应中的应用具有重要意义。对7LiH在高压等熵压缩下的可压缩性进行了实验和理论研究。利用j -100型磁累积发生器和x射线闪光照相技术,建立了低密度材料准等熵压缩实验技术。获得了动态闪光照相实验中样品目标的x射线图像和提取界面。根据压缩前后靶材的各个界面尺寸,得到7LiH与基准材料铝的压缩比。参考物的密度和利用其已知的等熵曲线提供参考物中的压力。7LiH内的压力由参考压力和计算的梯度校正系数推导而来。实验得到了438 GPa的准等熵数据点。利用mie - gren - neisen- debye理论,结合文献中的实验数据,构造了7LiH的半经验三项完全状态方程,并对其进行了验证。拟等熵数据点与理论结果基本一致。准等熵实验技术和结果拓宽了现有的研究范围,对进一步验证理论模型具有实用价值。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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