Pulsed Spark Discharge in Deionized Water for Nanoparticle Synthesis: Electrical Measurement and Cavitation Bubble Study

A. Dorval, K. Géraud, A. Hamdan, F. Valensi
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Abstract

Electrical discharges in dielectric liquids are considered as an efficient and eco-friendly technique for nanoparticle synthesis via controlled erosion of electrode. Understanding of mechanisms in the discharge and plasma-electrode interactions are needed to improve the efficiency of nanoparticles synthesis. In this study, we used a homemade pulsed power supply to produce spark discharges in deionized water with different electrodes, namely Cu, Al, and Steel. Voltage and current waveforms are acquired for discharges with various inter-electrode distances and applied voltages. The data is processed to report some characteristics of the discharges, such as breakdown voltage, discharge delay, injected charge, and energy. Also, we used a fast camera to visualize the dynamics of the post-discharge cavitation bubble. A relationship has been established between the discharge characteristics and the bubble dynamics; we found that higher is the injected energy larger is the bubble radius.
去离子水脉冲火花放电用于纳米粒子合成:电测量和空化泡研究
电介质液体中的放电被认为是一种高效且环保的通过控制电极侵蚀来合成纳米颗粒的技术。为了提高纳米粒子的合成效率,需要了解放电和等离子体电极相互作用的机制。在本研究中,我们使用自制的脉冲电源,在去离子水中使用不同的电极,即铜、铝和钢,产生火花放电。在不同的电极间距和施加电压下获得放电的电压和电流波形。对数据进行处理,以报告放电的一些特性,如击穿电压、放电延迟、注入电荷和能量。此外,我们使用快速相机来可视化放电后空化泡的动力学。建立了放电特性与气泡动力学之间的关系;我们发现,注入能量越高,气泡半径越大。
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