Microwave Properties of Bi2223 Thick Films on Ba(Sn, Mg, Ta)O3 Dielectric Disk

A. Oota, Daiki Washimoto, N. Kato, Y. Kintaka
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Abstract

We fabricated 2.1GHz TM010-mode microwave resonators with (Bi, Pb)2Sr2Ca2Cu3Ox (Bi2223) superconducting thick films on a Ba(Sn, Mg, Ta)O3 dielectric disk with a relative dielectric constant of er=24. The Bi2223 thick films were screen-printed on both sides of the dielectric disk and subjected to a double repetition of cold isostatic pressing at 0.4GPa and sintering at various temperatures ranging from 820 to 840°C. An increase of the sintering temperature raises the Bi2223 phase purity up to 98% on the surfaces of the thick films, but high-temperature sintering above 830°C causes a chemical reaction at the interface between the Bi2223 thick film and the dielectric disk. An optimization of the sintering temperature to 830°C gives the unloaded quality factors Qu as much as 74, 000 at 70K and 158, 000 at 25K, which correspond to surface resistances Rs of 0.34 and 0.15mΩ for Bi2223 thick films, respectively. These values are approximately 20 times higher than those for the resonator using Ag electrodes with the same structure.
Ba(Sn, Mg, Ta)O3介质盘上Bi2223厚膜的微波特性
采用(Bi, Pb)2Sr2Ca2Cu3Ox (Bi2223)超导厚膜,在相对介电常数为er=24的Ba(Sn, Mg, Ta)O3介质盘上制备了2.1GHz tm010模式微波谐振器。在介质盘两侧丝网印刷Bi2223厚膜,在0.4GPa下进行冷等静压,并在820 ~ 840℃的不同温度下进行两次重复烧结。升高烧结温度可使厚膜表面的Bi2223相纯度达到98%,但高于830℃的高温烧结会在Bi2223厚膜与介电盘的界面处发生化学反应。将烧结温度优化到830°C,在70K和25K下,卸载质量因子Qu分别高达74,000和158,000,对应于Bi2223厚膜的表面电阻Rs分别为0.34和0.15mΩ。这些值比使用相同结构的银电极的谐振器高约20倍。
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