Study of radium content and radon exhalation rates in raw building materials used in southern India

Abstract

As a potential source of indoor radiation arising from radon, a range of building materials (white cement, gray cement, gravel, gypsum, granite, marble, vitrified tile, and brick) were studied for the specific activity of radium and radon gas exhalation rates. The activity of radium was determined using scintillation gamma-ray spectrometry. Exhalation rates were assessed using passive and active measurement methods. Radon mass exhalation rates from powdered building materials and radon surface exhalation rates from slab-type building materials were measured. Activity concentrations of ²²⁶Ra in powder and slab-type building materials were found in the range of (1.12 – 14.98) Bqkg⁻¹ and (17 – 308) Bqkg⁻¹, respectively. ²²²Rn mass exhalation rates (mBqkg⁻¹h⁻¹) from the building materials were in the range of 15.0 ± 0.8 (gray cement) to 1.1 ± 0.1 (gravel). Surface exhalation rates (mBqm⁻²h⁻¹) for slab-type materials have a range of 317 ± 9 (brick) to 8 ± 2 (marble). Strong positive correlations were found between the specific activity of radium and radon mass exhalation rates (r = 0.9408) and radon surface exhalation rates (r = 0.7167) for building materials investigated. Obtained data indicates that the building materials used influence indoor radon concentration in dwellings.