Purification of fuel ethanol engine exhaust with platinum-loaded Ce0.5Zr0.5O2 catalyst

IF 3.1 3区 材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY
Fei Zhao, Chunyu Wang, Xianjing Liu, Qingyue Luo, Ling Zhu
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引用次数: 0

Abstract

This work aimed at exploring a new kind of purification catalysts for fuel ethanol engine exhaust. Platinum loaded on Ce0.5Zr0.5O2 was prepared by impregnation method and characterized by X-ray diffraction, Brunner–Emmet–Teller measurements (BET), temperature-programmed reduction of hydrogen, scanning electron microscope, and X-ray photoelectron spectra. The three-way catalyst platinum/ceria–zirconia/fw is prepared with the paste ball mill coating technique. And the catalytic performance is evaluated under simulated fuel ethanol engine exhaust gas condition. The catalysts not only show excellent low-temperature performances and several-way catalytic activities for carbon monoxide, hydrocarbons, nitrogen oxides, and acetaldehyde but also have better high-temperature resistance. The addition of sulfur dioxide to feedstream degrades the performances of the catalysts.
载铂Ce0.5Zr0.5O2催化剂净化燃料乙醇发动机尾气
本工作旨在探索一种新型的燃料乙醇发动机尾气净化催化剂。采用浸渍法制备了Ce0.5Zr0.5O2负载铂,并用x射线衍射、brunner - emet - teller测量(BET)、程序升温还原氢、扫描电镜和x射线光电子能谱对其进行了表征。采用膏体球磨机包覆技术制备了铂/二氧化锆/fw三元催化剂。并在模拟燃料乙醇发动机尾气工况下对其催化性能进行了评价。该催化剂不仅对一氧化碳、碳氢化合物、氮氧化物和乙醛具有优异的低温性能和多向催化活性,而且具有较好的耐高温性能。在进料流中加入二氧化硫会降低催化剂的性能。
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来源期刊
Nanomaterials and Nanotechnology
Nanomaterials and Nanotechnology NANOSCIENCE & NANOTECHNOLOGY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
7.20
自引率
21.60%
发文量
13
审稿时长
15 weeks
期刊介绍: Nanomaterials and Nanotechnology is a JCR ranked, peer-reviewed open access journal addressed to a cross-disciplinary readership including scientists, researchers and professionals in both academia and industry with an interest in nanoscience and nanotechnology. The scope comprises (but is not limited to) the fundamental aspects and applications of nanoscience and nanotechnology
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