Transient superconductivity without superconductivity

Abstract

Recent experiments on ${\mathrm{K}}_{3}{\mathrm{C}}_{60}$ and layered copper-oxide materials have reported substantial changes in the optical response following application of an intense THz pulse. These data have been interpreted as the stimulation of a transient superconducting state even at temperatures well above the equilibrium transition temperature. We propose an alternative phenomenology based on the assumption that the pulse creates a nonsuperconducting, though nonequilibrium, situation in which the linear response conductivity is negative. The negative conductivity implies that the spatially uniform prepulse state is unstable and evolves to a new state with a spontaneous electric polarization. This state exhibits coupled oscillations of entropy and electric charge whose coupling to incident probe radiation modifies the reflectivity, leading to an apparently superconductinglike response that resembles the data. Dependencies of the reflectivity on polarization and angle of incidence of the probe are predicted and other experimental consequences are discussed.