Laser-based double photoemission spectroscopy at surfaces

IF 8.7 2区 工程技术 Q1 CHEMISTRY, PHYSICAL
Cheng-Tien Chiang , Andreas Trützschler , Michael Huth , Robin Kamrla , Frank O. Schumann , Wolf Widdra
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引用次数: 9

Abstract

The recent development of double photoemission (DPE) spectroscopy at surfaces using laser-based high-order harmonic generation in combination with time-of-flight electron spectroscopy is reviewed. Relevant experimental conditions including the solid angle for collecting photoelectron pairs, the energy and angular resolutions, as well as the repetition rate and the photon energy range of light sources are introduced. As examples, we provide an overview of laser-based DPE results on the noble metals Ag and Cu as well as transition metal oxides NiO and CoO. The DPE energy and angular distributions of photoelectron pairs are compared with emphasis on the possible indications of electron-electron interaction. Potential further developments including femtosecond time-resolved DPE experiments are outlined.

基于激光的表面双光发射光谱
综述了基于激光的高次谐波产生与飞行时间电子能谱相结合的表面双光电发射光谱研究的最新进展。介绍了收集光电子对的立体角、能量和角分辨率、光源的重复率和光子能量范围等相关实验条件。作为例子,我们概述了基于激光的贵金属Ag和Cu以及过渡金属氧化物NiO和CoO的DPE结果。比较了光电子对的DPE能量和角分布,重点讨论了电子-电子相互作用的可能指示。概述了包括飞秒时间分辨DPE实验在内的潜在进一步发展。
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来源期刊
Progress in Surface Science
Progress in Surface Science 工程技术-物理:凝聚态物理
CiteScore
11.30
自引率
0.00%
发文量
10
审稿时长
3 months
期刊介绍: Progress in Surface Science publishes progress reports and review articles by invited authors of international stature. The papers are aimed at surface scientists and cover various aspects of surface science. Papers in the new section Progress Highlights, are more concise and general at the same time, and are aimed at all scientists. Because of the transdisciplinary nature of surface science, topics are chosen for their timeliness from across the wide spectrum of scientific and engineering subjects. The journal strives to promote the exchange of ideas between surface scientists in the various areas. Authors are encouraged to write articles that are of relevance and interest to both established surface scientists and newcomers in the field.
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