High-Accuracy Classification of Peanut Origin via Feature-Level Fusion of Multimodal Spectroscopy

IF 2 4区 化学 Q1 SOCIAL WORK
Wenlong Su, Limin Suo, Lili Qian, Zhaowei Wang
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引用次数: 0

Abstract

The geographical origin of peanuts directly determines their quality and market value. To overcome the destructive and time-consuming nature of conventional detection methods, this study proposes a novel nondestructive traceability strategy by integrating near-infrared (NIR) spectroscopy and low-field nuclear magnetic resonance (LF-NMR). Whole kernels of the peanut cultivar “LuhuaNo.9” were examined, from which NIR spectra reflecting chemical composition and LF-NMR signals characterizing moisture–lipid dynamics were simultaneously acquired. Two fusion strategies combined with several classifiers were evaluated: (1) low-level fusion, in which the original NIR and LF-NMR spectra were concatenated and modeled using support vector machine (SVM), extreme gradient boosting (XGBoost), random forest (RF), and a self-designed squeeze-and-excitation convolutional neural network (SE-CNN); (2) feature-level fusion, where informative spectral variables were selected using competitive adaptive reweighted sampling (CARS) to eliminate redundancy and noise. The results demonstrate that multisource data fusion substantially outperforms single-modality analysis, and the SE-CNN exhibits superior discriminatory ability compared with traditional machine learning models. In particular, the combination of CARS-based feature-level fusion and the SE-CNN achieved 100% classification accuracy on the test set, highlighting its outstanding performance. Overall, this work establishes a high-precision traceability strategy that integrates multidimensional spectral information with deep learning, markedly improving identification efficiency while preserving sample integrity. The proposed approach holds significant promise for the protection of geographical indications and quality monitoring of agricultural products.

基于多模态光谱特征级融合的花生产地高精度分类
花生的产地直接决定了花生的品质和市场价值。为了克服传统检测方法的破坏性和耗时性,本研究提出了一种将近红外(NIR)光谱和低场核磁共振(LF-NMR)相结合的新型无损溯源策略。花生品种“芦花野”的全粒。研究了9英寸,同时获得了反映化学成分的近红外光谱和表征水分-脂质动力学的LF-NMR信号。评估了两种结合多种分类器的融合策略:(1)低水平融合,将原始NIR和LF-NMR光谱连接起来,并使用支持向量机(SVM)、极端梯度增强(XGBoost)、随机森林(RF)和自行设计的压缩激励卷积神经网络(SE-CNN)建模;(2)特征级融合,利用竞争自适应重加权采样(CARS)选择信息丰富的光谱变量,消除冗余和噪声。结果表明,多源数据融合大大优于单模态分析,并且SE-CNN与传统机器学习模型相比具有优越的区分能力。特别是将基于cars的特征级融合与SE-CNN相结合,在测试集上实现了100%的分类准确率,突出了其出色的性能。总体而言,本研究建立了一种高精度的可追溯策略,将多维光谱信息与深度学习相结合,在保持样本完整性的同时显著提高了识别效率。该方法对地理标志保护和农产品质量监测具有重要意义。
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来源期刊
Journal of Chemometrics
Journal of Chemometrics 化学-分析化学
CiteScore
5.20
自引率
8.30%
发文量
78
审稿时长
2 months
期刊介绍: The Journal of Chemometrics is devoted to the rapid publication of original scientific papers, reviews and short communications on fundamental and applied aspects of chemometrics. It also provides a forum for the exchange of information on meetings and other news relevant to the growing community of scientists who are interested in chemometrics and its applications. Short, critical review papers are a particularly important feature of the journal, in view of the multidisciplinary readership at which it is aimed.
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