Site-Specific Calibration of Low-Cost Particulate Matter (PM) 2.5 Monitors in the United States: A Comparison of Industrial and Non-Industrial Communities.

IF 2.5 4区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES
Aerosol and Air Quality Research Pub Date : 2026-01-01 Epub Date: 2026-03-25 DOI:10.1007/s44408-026-00112-7
Jung Hyun Lee, Subin Han, Chang Geun Lee, Tim DaSilva, Carolina Gonzalez-Canas, Jon-Paul McCool, Kenneth L Brown, Jodi Allen, Graham F Peaslee, Jae Hong Park, Julie Peller, Christopher R Iceman, Ellen M Wells
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引用次数: 0

Abstract

Particulate matter (PM) poses a significant public health concern, particularly in industrialized communities. While modern sophisticated air monitors like those deployed by the United States Environmental Protection Agency (US EPA) provide accurate 24-h PM2.5 (PM ≤ 2.5 µm) data, limited spatial and temporal coverage may create monitoring gaps. Low-cost monitors, such as a PurpleAir monitor (PA-II), offer an accessible alternative; however, their accuracy can be influenced by local environmental conditions and PM characteristics. This study evaluated the site-specific performance of PA-II in an industrial region within northern Lake County (N = 6) and a suburban region of Tippecanoe County (N = 4), both in Indiana, United States. As a reference measurement, a deployable particulate sampler (DPS) was co-located with each PA-II. For microscopic analysis, PM was collected on a glass substrate. PA-II data were assessed in raw form and following calibration using two methods, with performance assessed by root mean square error (RMSE) and the coefficient of determination (R2). Microscopic analysis revealed the presence of dark, irregular particles near industrial sites in northern Lake County, which may affect sensor readings by altering light-scattering efficiency. Raw PA-II data showed weak absolute agreement with DPS measurements in northern Lake County (RMSE: 2.04 µg/m3, R2: 0.25), while the US-wide calibration exhibited the best performance (RMSE: 1.40 µg/m3; R2: 0.67). In contrast, raw data showed the best performance in Tippecanoe County (RMSE: 0.62 µg/m3; R2: 0.94). These findings highlight the relevance of site-specific calibration approaches to enhance the accuracy of low-cost PM2.5 monitors, especially in environmentally impacted communities.

Graphical abstract:

Supplementary information: The online version contains supplementary material available at 10.1007/s44408-026-00112-7.

Abstract Image

Abstract Image

Abstract Image

美国低成本颗粒物(PM) 2.5监测仪的定点校准:工业和非工业社区的比较。
颗粒物(PM)是一个重大的公共卫生问题,特别是在工业化社区。虽然像美国环境保护署(US EPA)部署的现代精密空气监测仪可以提供精确的24小时PM2.5 (PM≤2.5µm)数据,但有限的空间和时间覆盖可能会造成监测空白。低成本监视器,如PurpleAir监视器(PA-II),提供了一个可访问的替代方案;然而,它们的准确性会受到当地环境条件和PM特征的影响。本研究评估了美国印第安纳州Lake县北部的一个工业区(N = 6)和Tippecanoe县的一个郊区(N = 4)中PA-II的场地特异性性能。作为参考测量,可展开颗粒采样器(DPS)与每个PA-II一起放置。为了进行显微分析,PM被收集在玻璃基板上。采用两种方法对原始形式和校正后的PA-II数据进行评估,以均方根误差(RMSE)和决定系数(R2)评估其性能。显微镜分析显示,在莱克县北部的工业基地附近存在黑色的不规则颗粒,这可能通过改变光散射效率来影响传感器读数。原始PA-II数据与Lake县北部的DPS测量结果的绝对一致性较弱(RMSE: 2.04µg/m3, R2: 0.25),而美国范围的校准表现出最好的性能(RMSE: 1.40µg/m3, R2: 0.67)。原始数据显示,Tippecanoe县的表现最佳(RMSE: 0.62µg/m3; R2: 0.94)。这些发现强调了特定地点校准方法的相关性,以提高低成本PM2.5监测仪的准确性,特别是在受环境影响的社区。图片摘要:补充资料:在线版本包含补充资料,网址为10.1007/s44408-026-00112-7。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
Aerosol and Air Quality Research
Aerosol and Air Quality Research ENVIRONMENTAL SCIENCES-
CiteScore
8.30
自引率
10.00%
发文量
163
审稿时长
3 months
期刊介绍: The international journal of Aerosol and Air Quality Research (AAQR) covers all aspects of aerosol science and technology, atmospheric science and air quality related issues. It encompasses a multi-disciplinary field, including: - Aerosol, air quality, atmospheric chemistry and global change; - Air toxics (hazardous air pollutants (HAPs), persistent organic pollutants (POPs)) - Sources, control, transport and fate, human exposure; - Nanoparticle and nanotechnology; - Sources, combustion, thermal decomposition, emission, properties, behavior, formation, transport, deposition, measurement and analysis; - Effects on the environments; - Air quality and human health; - Bioaerosols; - Indoor air quality; - Energy and air pollution; - Pollution control technologies; - Invention and improvement of sampling instruments and technologies; - Optical/radiative properties and remote sensing; - Carbon dioxide emission, capture, storage and utilization; novel methods for the reduction of carbon dioxide emission; - Other topics related to aerosol and air quality.
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