High-Efficiency Aqueous Zinc-ion Capacitors Based On Mofs/cofs-derived Nanomaterials: Challenges and Future Prospects

IF 3.2 4区化学 Q3 CHEMISTRY, PHYSICAL

Electrocatalysis Pub Date : 2025-12-19 DOI:10.1007/s12678-025-00997-9

Xuexue Pan, Yi Zhao, Huiling Zhou, Jianhui Zhang

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引用次数: 0

Abstract

Aqueous zinc-ion capacitors have garnered significant attention recently due to their safety, environmental benefits, and high capacity. However, its practical application still faces many challenges. Metal–organic frameworks (MOFs) and Covalent organic frameworks (COFs)-derived nanomaterials have demonstrated outstanding potential as electrode materials due to their unique structure and adjustable properties. Here, the current application status of MOFs/COFs-derived nanomaterials in high-efficiency aqueous ZICs is reviewed and the structure and properties of these materials, as well as their synthesis methods and advantages in capacitors are explored. The key factors influencing the properties of aqueous ZICs, including material structure, morphology, electrochemical characteristics, stability, and cycle life, are further examined. Although there are current challenges in the controllability of material preparation, large-scale production, electrolyte and electrode interface, the future development of aqueous ZICs is promising through new material design and synthesis strategies, performance optimization, and interdisciplinary research. This paper examines the future research directions and application potential of MOFs/COFs-derived nanomaterials in waterborne ZICs.

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基于Mofs/cofs衍生纳米材料的高效水性锌离子电容器：挑战与未来展望

水性锌离子电容器由于其安全、环保和高容量等优点，近年来受到了广泛的关注。但其实际应用仍面临诸多挑战。金属有机骨架（MOFs）和共价有机骨架（COFs）衍生的纳米材料由于其独特的结构和可调节的性能，在电极材料方面表现出了突出的潜力。本文综述了MOFs/ cofs衍生纳米材料在高效水性ZICs中的应用现状，探讨了mfs / cofs衍生纳米材料的结构和性能，以及它们在电容器中的合成方法和优势。进一步研究了影响水性ZICs性能的关键因素，包括材料结构、形貌、电化学特性、稳定性和循环寿命。尽管目前在材料制备的可控性、大规模生产、电解质和电极界面等方面存在挑战，但通过新的材料设计和合成策略、性能优化和跨学科研究，水性ZICs的未来发展前景广阔。展望了mof / cofs衍生纳米材料在水性复合材料中的研究方向和应用潜力。

本文章由计算机程序翻译，如有差异，请以英文原文为准。

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来源期刊

Electrocatalysis CHEMISTRY, PHYSICAL-ELECTROCHEMISTRY

CiteScore

4.80

自引率

6.50%

发文量

审稿时长

>12 weeks

期刊介绍： Electrocatalysis is cross-disciplinary in nature, and attracts the interest of chemists, physicists, biochemists, surface and materials scientists, and engineers. Electrocatalysis provides the unique international forum solely dedicated to the exchange of novel ideas in electrocatalysis for academic, government, and industrial researchers. Quick publication of new results, concepts, and inventions made involving Electrocatalysis stimulates scientific discoveries and breakthroughs, promotes the scientific and engineering concepts that are critical to the development of novel electrochemical technologies. Electrocatalysis publishes original submissions in the form of letters, research papers, review articles, book reviews, and educational papers. Letters are preliminary reports that communicate new and important findings. Regular research papers are complete reports of new results, and their analysis and discussion. Review articles critically and constructively examine development in areas of electrocatalysis that are of broad interest and importance. Educational papers discuss important concepts whose understanding is vital to advances in theoretical and experimental aspects of electrochemical reactions.