Multifunctional MXene/GO/rGO-Textile Flexible Sensor with Outstanding Electrothermal and Strain-Sensing Performance for Wearable Applications

Abstract

To address the inherent limitations of easy oxidation and unstable electrical properties in two-dimensional MXene-based flexible sensors, this study developed a MXene/GO/rGO (reduced graphene oxide) textile-based flexible sensor using a lamination method and in situ steam reduction technology. The sensor was constructed on a high-elasticity knitted polyester fabric, with MXene as the primary conductive layer, graphene oxide (GO) as the adhesive layer, and reduced graphene oxide (rGO) as the protective encapsulation surface layer. The tensile strain-sensing and electrothermal properties of the resulting e-textile were systematically characterized. The MXene/GO/rGO textile demonstrated outstanding electrical and mechanical performance, achieving a conductivity of 39.7 S·m−1, a gauge factors ranging from –3 to –1.6, and a controllable electrothermal heating range from 43 °C to 85 °C under currents of 0.02–0.05 A. Experimental results demonstrated that under applied currents of 0.02, 0.03, 0.04, and 0.05 A, the fabric reached temperatures of 43, 56, 73, and 85 °C, respectively, and remained constant over extended periods. In terms of strain sensing, the sensor exhibited a short response time (65 ms), high discriminability for different strain levels and stretching rates, and a consistent relative resistance change (ΔR/R0) under various stretching speeds (0.5, 1, 2, 4, and 6 mm/s). Compared with sensors based on a single conductive material, the MXene/GO/rGO polyester fabric sensor shows superior electrothermal and strain-sensing performance, indicating promising potential for applications in intelligent wearable textiles such as medical thermal therapy, sports monitoring, and health management.