Competing Magnetic States in the Possible Altermagnet Candidate GdAlGe.

Abstract

Altermagnetism, a newly discovered magnetic order, combines zero net magnetization with nonrelativistic spin splitting of electronic bands. Its ability to utilize the advantages of both antiferromagnets and ferromagnets is highly promising for spintronic applications. Currently, the merge of altermagnetism and weak ferromagnetism in a single material excites significant interest as it provides additional control mechanisms over material properties. However, the role of dimensionality in this interplay is yet to be explored. Here, we study magnetism and electron transport in epitaxial films of the candidate altermagnet GdAlGe ranging from bulk-like to a single monolayer. The films exhibit the anomalous Hall effect and negative magnetoresistance. In contrast to altermagnetic GdAlSi, the candidate altermagnet GdAlGe demonstrates an admixture of the ferromagnetic state whose contribution increases as the system approaches the 2D limit. The coexistence of the magnetic states induces technologically important intrinsic exchange bias. The present work underpins future studies and applications of nanoscale altermagnets.