A novel retrieval of global dust optical depth and effective diameter based on MODIS thermal infrared observations

Abstract

Airborne mineral dust significantly influences Earth's climate through perturbing Earth's radiation budget, modulating cloud formation and microphysical properties, and fertilizing the biosphere. Recent field campaigns have revealed substantially more coarse-mode dust particles in the atmosphere than previously recognized, yet current satellite retrievals and climate models inadequately represent these particles. This study presents a novel retrieval algorithm for dust aerosol optical depth at 10 μm (AOD_10μm) and effective diameter (Deff) using Moderate Resolution Imaging Spectroradiometer (MODIS) thermal infrared (TIR) observations over global land and ocean. Building upon the previous synergistic approach for MODIS and the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP), we improve the retrieval from CALIOP-track-limited coverage to full-swath MODIS observations at 10-km resolution over both ocean and land surfaces. The retrieval improvements include: (1) application of climatological CALIOP dust vertical profiles (2007–2017) to constrain dust vertical distribution for off-CALIOP-track pixels; (2) the improved optimization method to effectively handle non-monotonic cost functions arising from temperature inversions within the Saharan Air Layer; and (3) extension to land surfaces through incorporation of MODIS-retrieved surface emissivity and ERA5 reanalysis data. Validation against coarse-mode AOD from global AERONET (N = 4703) and MAN (N = 1673) observations yields R = 0.82 and 0.85 for AOD_10μm, with retrieval uncertainty characterized as ε = 15 % × AOD + 0.04. The retrieved Deff demonstrates excellent agreement with in-situ measurements collected from 24 field campaigns around the globe (R = 0.84, MBE = 0.23 μm, RMSE = 0.73 μm), capturing the particle size variation from near-source regions (Deff = 7–8 μm) to long-range transport (Deff = 3–5 μm). Case studies of dust events over the Namibian coast and trans-Atlantic corridor demonstrate the retrieval's capability to resolve episodic dust properties and size-dependent deposition during transport. This improved retrieval addresses the critical observational gap for coarse and super-coarse dust particles (D > 5 μm), providing essential constraints for dust life cycle studies and climate model evaluation.