Intense Photoluminescence in Erbium-Ion-Implanted Lithium Niobate Thin Films and Its Interplay with Lattice Defects

IF 7.2 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY
Liangling Wang, Sören Lerner, Houbin Zhu, Xiaojun Cui, Binge Zeng, Fengkai Wei, Elke Wendler, Carsten Ronning
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Abstract

Erbium-doped lithium niobate on insulator (Er-LNOI) has attracted significant attention for its potential in integrated photonics and quantum applications due to its efficient 1540 nm emission in the telecom band. In this work, the lattice damage and infrared photoluminescence of Er-LNOI fabricated via Er ion implantation and subsequent thermal annealing is investigated. Damage profiles are analyzed using Rutherford backscattering spectrometry in channeling mode (RBS/C), revealing the formation of an amorphous layer during ion implantation. However, re-crystallization into an Er-doped LNOI single crystal occurs with some remaining dislocation loops after annealing. Photoluminescence measurements at room temperature demonstrate intense infrared emission with no evidence of Er clustering and concentration quenching up to an Er fluence of 2.63 × 101⁵ ions cm2. Power- and temperature-dependent PL spectra suggest stable emission and distinct thermal quenching mechanisms for the two Stark-split transitions. The results confirm the effective optical activation of single crystalline Er-LNOI and highlight its promise for on-chip light sources and active photonic devices.

Abstract Image

铒离子注入铌酸锂薄膜的强光致发光及其与晶格缺陷的相互作用
绝缘体上掺铒铌酸锂(Er-LNOI)由于其在电信波段的1540 nm高效发射,在集成光子学和量子应用中具有很大的潜力。本文研究了铒离子注入和热退火法制备的铒- lnoi的晶格损伤和红外光致发光特性。利用通道模式(RBS/C)下的卢瑟福后向散射光谱分析了损伤谱,揭示了离子注入过程中非晶层的形成。退火后,再结晶成掺杂铒的LNOI单晶,并留下了一些位错环。室温下的光致发光测量显示出强烈的红外发射,没有证据表明Er聚集和浓度猝灭,Er的影响高达2.63 × 101个5离子cm2。功率和温度相关的PL光谱表明两个stark分裂跃迁的稳定发射和不同的热猝灭机制。结果证实了单晶Er-LNOI的有效光学激活,并强调了其在片上光源和有源光子器件中的应用前景。
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来源期刊
Advanced Optical Materials
Advanced Optical Materials MATERIALS SCIENCE, MULTIDISCIPLINARY-OPTICS
CiteScore
13.70
自引率
6.70%
发文量
883
审稿时长
1.5 months
期刊介绍: Advanced Optical Materials, part of the esteemed Advanced portfolio, is a unique materials science journal concentrating on all facets of light-matter interactions. For over a decade, it has been the preferred optical materials journal for significant discoveries in photonics, plasmonics, metamaterials, and more. The Advanced portfolio from Wiley is a collection of globally respected, high-impact journals that disseminate the best science from established and emerging researchers, aiding them in fulfilling their mission and amplifying the reach of their scientific discoveries.
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