Hybrid Lithium Electrolytes as Potential Electrolytes for Energy Storage Devices: A Pathway to Sustainable and High-Efficiency Solutions

IF 3 3区化学 Q2 CHEMISTRY, APPLIED

Topics in Catalysis Pub Date : 2025-07-29 DOI:10.1007/s11244-025-02154-4

Chitra Sharma, Harpreet Kaur, Abhinay Thakur, Ramesh Chand Thakur, Harmanjit Singh Dosanjh

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Abstract

The urgent demand for high-performance and sustainable energy storage solutions necessitates the development of advanced electrolytes with superior electrochemical properties. Hybrid lithium electrolytes, which integrate the advantages of inorganic and organic ionic conductors, have emerged as promising candidates for next-generation energy storage devices. This review presents a comprehensive bibliometric analysis of 1569 research articles from 2019 to 2024, sourced from Scopus and Web of Science (WOS) databases, highlighting the rising research focus on hybrid electrolytes. Key material properties such as wide electrochemical windows, thermal and chemical stability, low toxicity, and reduced volatility are critical for enhancing battery performance. The discussion encompasses recent advancements in solid-state, polymer, and hybrid electrolytes, emphasizing their role in improving energy density, cycling stability, and safety. Furthermore, this study examines the challenges associated with hybrid electrolytes, including ionic conductivity limitations, interfacial compatibility, and scalability for industrial applications. The integration of novel materials such as NASICON-type ceramics, perovskites, sulfides, and garnet-based electrolytes is explored for their potential to revolutionize lithium-ion battery technologies. By bridging the gap between fundamental research and practical implementation, this review provides insights into the future directions of hybrid electrolytes, paving the way for more efficient and sustainable energy storage systems.

Graphical Abstract

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混合锂电解质作为储能装置的潜在电解质：通往可持续和高效解决方案的途径

对高性能和可持续能源存储解决方案的迫切需求要求开发具有优异电化学性能的先进电解质。混合锂电解质集成了无机和有机离子导体的优点，已成为下一代储能设备的有前途的候选者。本文对2019年至2024年的1569篇研究论文进行了全面的文献计量分析，这些论文来自Scopus和Web of Science （WOS）数据库，突出了对混合电解质的研究日益关注。关键的材料特性，如宽电化学窗口、热稳定性和化学稳定性、低毒性和减少挥发性，对提高电池性能至关重要。讨论涵盖了固态、聚合物和混合电解质的最新进展，强调了它们在提高能量密度、循环稳定性和安全性方面的作用。此外，本研究还探讨了与混合电解质相关的挑战，包括离子电导率限制、界面兼容性和工业应用的可扩展性。新材料如nasicon型陶瓷、钙钛矿、硫化物和石榴石基电解质的整合，探索了它们革新锂离子电池技术的潜力。通过弥合基础研究和实际应用之间的差距，本综述为混合电解质的未来发展方向提供了见解，为更高效和可持续的能源存储系统铺平了道路。图形抽象

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来源期刊

Topics in Catalysis 化学-物理化学

CiteScore

5.70

自引率

5.60%

发文量

197

审稿时长

2 months

期刊介绍： Topics in Catalysis publishes topical collections in all fields of catalysis which are composed only of invited articles from leading authors. The journal documents today’s emerging and critical trends in all branches of catalysis. Each themed issue is organized by renowned Guest Editors in collaboration with the Editors-in-Chief. Proposals for new topics are welcome and should be submitted directly to the Editors-in-Chief. The publication of individual uninvited original research articles can be sent to our sister journal Catalysis Letters. This journal aims for rapid publication of high-impact original research articles in all fields of both applied and theoretical catalysis, including heterogeneous, homogeneous and biocatalysis.