Glass–water interactions: From surface into the bulk

IF 3.8 3区材料科学 Q1 MATERIALS SCIENCE, CERAMICS

Journal of the American Ceramic Society Pub Date : 2025-07-30 DOI:10.1111/jace.70137

Yen-Ting Lin, Mohammad Naghashnejad, Ava N. Zoba, Andrew L. Ogrinc, Collin J. Wilkinson, Mason M. Link, Yiwen Guo, John C. Mauro, Seong H. Kim

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Abstract

This article provides a comprehensive review of the intricate interactions between water and glass, which significantly alter not only the chemical properties of glass surface but also its mechanical properties. These interactions impact adhesion, contact mechanics, and corrosion—key factors for industrial and technological applications. Encompassing studies from various advanced characterization techniques and computational simulations, the review delves into mechanisms such as physisorption and chemisorption, the molecular behavior of water at glass interfaces, and the effects of water ingress on glass network structure. By identifying critical knowledge gaps and unresolved questions, this work highlights future research needs. The findings have implications on glass durability and performance in industrial applications, from nuclear waste containment to consumer electronics, offering pathways to engineer glass materials with enhanced resistance to environmental degradation.

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玻璃-水相互作用：从表面到体

本文综述了水与玻璃之间复杂的相互作用，这些相互作用不仅显著地改变了玻璃表面的化学性质，而且显著地改变了玻璃表面的力学性能。这些相互作用影响着附着力、接触力学和腐蚀——工业和技术应用的关键因素。包括各种先进表征技术和计算模拟的研究，综述深入研究了物理吸附和化学吸附等机制，水在玻璃界面的分子行为，以及水进入对玻璃网络结构的影响。通过识别关键的知识差距和未解决的问题，这项工作突出了未来的研究需求。这些发现对玻璃在工业应用中的耐久性和性能有影响，从核废料容器到消费电子产品，为设计具有增强抗环境退化能力的玻璃材料提供了途径。

本文章由计算机程序翻译，如有差异，请以英文原文为准。

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来源期刊

Journal of the American Ceramic Society 工程技术-材料科学：硅酸盐

CiteScore

7.50

自引率

7.70%

发文量

590

审稿时长

2.1 months

期刊介绍： The Journal of the American Ceramic Society contains records of original research that provide insight into or describe the science of ceramic and glass materials and composites based on ceramics and glasses. These papers include reports on discovery, characterization, and analysis of new inorganic, non-metallic materials; synthesis methods; phase relationships; processing approaches; microstructure-property relationships; and functionalities. Of great interest are works that support understanding founded on fundamental principles using experimental, theoretical, or computational methods or combinations of those approaches. All the published papers must be of enduring value and relevant to the science of ceramics and glasses or composites based on those materials. Papers on fundamental ceramic and glass science are welcome including those in the following areas: Enabling materials for grand challenges[...] Materials design, selection, synthesis and processing methods[...] Characterization of compositions, structures, defects, and properties along with new methods [...] Mechanisms, Theory, Modeling, and Simulation[...] JACerS accepts submissions of full-length Articles reporting original research, in-depth Feature Articles, Reviews of the state-of-the-art with compelling analysis, and Rapid Communications which are short papers with sufficient novelty or impact to justify swift publication.