Levels of elements in road dust of Shillong, Northeast India: characterization, source apportionment and health risk assessment.

IF 3.8 3区 环境科学与生态学 Q3 ENGINEERING, ENVIRONMENTAL
Nicholas Khundrakpam, Biwel Binong, Rebekha Mushahary, Anamika Nath, Mebaaibok L Nonglait, Pratibha Deka
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Abstract

The study analyzed eleven elements in road dust from residential areas, traffic areas, commercial areas, and plastic paper and e-waste collection sites in Shillong, Northeast India. Elemental concentrations followed the order: Al > Fe > Mg > Mn > Zn > Pb > Cu > Cr > Co > Ni > Cd. Among these, Cd showed the highest enrichment (EF = 63.01), followed by Pb (EF = 24.78), and contributed 92% and 6% of the ecological risk, respectively. Pollution indices confirmed significant contamination in all sites. The geoaccumulation index (Igeo) indicated extreme pollution for Cd, moderate to extreme for Pb, and low to moderate levels for other elements. Strong positive correlations were observed among Al-Mg, Co-Cu, Co-Mn, Pb-Zn, and Pb-Cd, with moderate correlations (r = 0.4-0.6) for Cd-Zn, Cu-Zn, and Fe-Cr. PCA revealed three major sources: anthropogenic and crustal, traffic and e-waste, and geogenic. The hazard index exceeded 1 for children at all sites, indicating potential non-carcinogenic risk, primarily via ingestion. Chromium was the main contributor to cancer risk, though overall levels remained within safe limits. FTIR and PXRD analyses confirmed quartz as the dominant mineral, along with silicate, carbonate, and others. The study recommends pollution control measures to aid urban planning and safeguard public health.

印度东北部西隆道路粉尘中的元素水平:特征、来源分配和健康风险评估。
该研究分析了来自印度东北部西隆居民区、交通区、商业区以及塑料纸和电子垃圾收集场的道路粉尘中的11种元素。元素浓度跟随订单:艾尔>铁Mg > >锰>锌>铅>铜> Cr >有限公司>镍> Cd。其中,Cd的富集程度最高(EF = 63.01),其次是Pb (EF = 24.78),对生态风险的贡献率分别为92%和6%。污染指数证实所有地点都有严重污染。地质累积指数(Igeo)显示Cd为重度污染,Pb为中度至重度污染,其他元素为低至中度污染。Al-Mg、Co-Cu、Co-Mn、Pb-Zn和Pb-Cd呈正相关,Cd-Zn、Cu-Zn和Fe-Cr呈正相关(r = 0.4-0.6)。主成分分析揭示了3个主要来源:人为和地壳、交通和电子垃圾、地质。所有地点的儿童危害指数均超过1,表明主要通过摄入存在潜在的非致癌风险。铬是致癌风险的主要因素,尽管总体水平仍在安全范围内。FTIR和PXRD分析证实石英是主要矿物,还有硅酸盐、碳酸盐和其他矿物。该研究建议采取污染控制措施,以帮助城市规划和保障公众健康。
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来源期刊
Environmental Geochemistry and Health
Environmental Geochemistry and Health 环境科学-工程:环境
CiteScore
8.00
自引率
4.80%
发文量
279
审稿时长
4.2 months
期刊介绍: Environmental Geochemistry and Health publishes original research papers and review papers across the broad field of environmental geochemistry. Environmental geochemistry and health establishes and explains links between the natural or disturbed chemical composition of the earth’s surface and the health of plants, animals and people. Beneficial elements regulate or promote enzymatic and hormonal activity whereas other elements may be toxic. Bedrock geochemistry controls the composition of soil and hence that of water and vegetation. Environmental issues, such as pollution, arising from the extraction and use of mineral resources, are discussed. The effects of contaminants introduced into the earth’s geochemical systems are examined. Geochemical surveys of soil, water and plants show how major and trace elements are distributed geographically. Associated epidemiological studies reveal the possibility of causal links between the natural or disturbed geochemical environment and disease. Experimental research illuminates the nature or consequences of natural or disturbed geochemical processes. The journal particularly welcomes novel research linking environmental geochemistry and health issues on such topics as: heavy metals (including mercury), persistent organic pollutants (POPs), and mixed chemicals emitted through human activities, such as uncontrolled recycling of electronic-waste; waste recycling; surface-atmospheric interaction processes (natural and anthropogenic emissions, vertical transport, deposition, and physical-chemical interaction) of gases and aerosols; phytoremediation/restoration of contaminated sites; food contamination and safety; environmental effects of medicines; effects and toxicity of mixed pollutants; speciation of heavy metals/metalloids; effects of mining; disturbed geochemistry from human behavior, natural or man-made hazards; particle and nanoparticle toxicology; risk and the vulnerability of populations, etc.
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