Marzieh Hassanpour , Mehdi Hassanpour , MohammadReza Rezaie , Mohammad Rashed Iqbal Faruque
{"title":"The feasibility of calculating the enrichment of 235U using the PIGE method with high-energy protons","authors":"Marzieh Hassanpour , Mehdi Hassanpour , MohammadReza Rezaie , Mohammad Rashed Iqbal Faruque","doi":"10.1016/j.anucene.2025.111882","DOIUrl":null,"url":null,"abstract":"<div><div>In this study, an attempt has been made to investigate the <sup>235</sup>U enrichment percentage in uranium compounds using the PIGE method with 25 MeV proton energy and to calculate the characteristic gamma energy of <sup>235</sup>U. The results indicate that the characteristic gamma energy of 2.2 MeV corresponds to <sup>235</sup>U in the uranium compound, where no gamma line from <sup>238</sup>U is observed at this energy. By altering the percentage of <sup>235</sup>U enrichment in the compound, the response of the CsI(Tl) detector to the 2.2 MeV gamma is formulated as a function of different enrichment percentages, utilizing the results obtained from MCNPX simulations. Furthermore, by examining various nuclear processes resulting from the interaction of protons with <sup>235</sup>U and <sup>238</sup>U, the reason for the gamma radiation at 2.2 MeV for <sup>235</sup>U is also elucidated.</div></div>","PeriodicalId":8006,"journal":{"name":"Annals of Nuclear Energy","volume":"226 ","pages":"Article 111882"},"PeriodicalIF":2.3000,"publicationDate":"2025-09-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Annals of Nuclear Energy","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0306454925006991","RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"NUCLEAR SCIENCE & TECHNOLOGY","Score":null,"Total":0}
引用次数: 0
Abstract
In this study, an attempt has been made to investigate the 235U enrichment percentage in uranium compounds using the PIGE method with 25 MeV proton energy and to calculate the characteristic gamma energy of 235U. The results indicate that the characteristic gamma energy of 2.2 MeV corresponds to 235U in the uranium compound, where no gamma line from 238U is observed at this energy. By altering the percentage of 235U enrichment in the compound, the response of the CsI(Tl) detector to the 2.2 MeV gamma is formulated as a function of different enrichment percentages, utilizing the results obtained from MCNPX simulations. Furthermore, by examining various nuclear processes resulting from the interaction of protons with 235U and 238U, the reason for the gamma radiation at 2.2 MeV for 235U is also elucidated.
期刊介绍:
Annals of Nuclear Energy provides an international medium for the communication of original research, ideas and developments in all areas of the field of nuclear energy science and technology. Its scope embraces nuclear fuel reserves, fuel cycles and cost, materials, processing, system and component technology (fission only), design and optimization, direct conversion of nuclear energy sources, environmental control, reactor physics, heat transfer and fluid dynamics, structural analysis, fuel management, future developments, nuclear fuel and safety, nuclear aerosol, neutron physics, computer technology (both software and hardware), risk assessment, radioactive waste disposal and reactor thermal hydraulics. Papers submitted to Annals need to demonstrate a clear link to nuclear power generation/nuclear engineering. Papers which deal with pure nuclear physics, pure health physics, imaging, or attenuation and shielding properties of concretes and various geological materials are not within the scope of the journal. Also, papers that deal with policy or economics are not within the scope of the journal.