Menghan Jiang , Anamul Haq Mir , Mounib Bahri , Yingjie Zhang , Keith Arnold , Nigel Browning , Karl Whittle , Maulik Patel
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引用次数: 0
Abstract
Glass-ceramics have been regarded as potential nuclear wasteforms for immobilization of high-level waste. Understanding material modifications due to combined damage by α-decay is the key in predicting long-term evolution of wasteforms. 10 keV in-situ helium implantation experiments were carried out on TEM specimens extracted from Y2Ti2O7 glass-ceramic samples pre-irradiated with 7 MeV Au to understand the kinetics of helium bubble evolution, showing that the accumulation of He can lead to the nucleation of helium bubbles within the amorphous Y2Ti2O7 ceramic phase at a critical concentration of 3.4 at.%. Structural modifications by Au irradiation were characterized using grazing-incidence x-ray diffraction (GIXRD) and scanning transmission electron microscopy (STEM). The STEM results revealed that complete amorphization of the pyrochlore structure occurred at Au/cm2. A phase transformation to defect-fluorite structure is also observed at the irradiated interface. Besides, a potential Y-rich phase was identified within the glass matrix, which likely originated from the effects of irradiation.
期刊介绍:
The Journal of Nuclear Materials publishes high quality papers in materials research for nuclear applications, primarily fission reactors, fusion reactors, and similar environments including radiation areas of charged particle accelerators. Both original research and critical review papers covering experimental, theoretical, and computational aspects of either fundamental or applied nature are welcome.
The breadth of the field is such that a wide range of processes and properties in the field of materials science and engineering is of interest to the readership, spanning atom-scale processes, microstructures, thermodynamics, mechanical properties, physical properties, and corrosion, for example.
Topics covered by JNM
Fission reactor materials, including fuels, cladding, core structures, pressure vessels, coolant interactions with materials, moderator and control components, fission product behavior.
Materials aspects of the entire fuel cycle.
Materials aspects of the actinides and their compounds.
Performance of nuclear waste materials; materials aspects of the immobilization of wastes.
Fusion reactor materials, including first walls, blankets, insulators and magnets.
Neutron and charged particle radiation effects in materials, including defects, transmutations, microstructures, phase changes and macroscopic properties.
Interaction of plasmas, ion beams, electron beams and electromagnetic radiation with materials relevant to nuclear systems.