Assessing the Impact of Wildfire Smoke Transport Through Chemical Transport Modeling, Satellite Retrievals, and Ground-Based Observations of Ozone in Rural Nevada

Yi Ji*, Xiaodan Zhang, Abiola S. Lawal, Heather A. Holmes and Cesunica E. Ivey, 
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Abstract

Wildfires emit a large amount of ozone precursors, nitrogen oxides, and particulate matter into the troposphere and sometimes the stratosphere. With the increasing wildfire events in recent years, the western U.S. regions may experience challenges with higher-than-normal air pollution levels during the fire season (June-October). Therefore, determining the ozone enhancement pattern from wildfire smoke is crucial to understanding the influence of wildfire plume transport on a subregional basis. This study investigates the impact of the 2013 Rim Fire on ozone levels in rural Nevada, employing a combination of ground-based monitors, satellite remote sensing, and atmospheric modeling. The research focuses on understanding how wildfire smoke affects ozone concentrations in the downwind regions. Findings indicate significant ozone enhancements on smoke days compared to nonsmoke days, highlighting the contribution of wildfire emissions to regional air quality deterioration. The study demonstrates that the chemical transport model underestimated ozone levels downwind of wildfire plumes, likely due to uncertainties in smoke emissions estimates and differences in chemical mechanisms across model versions. Satellite observations of nitrogen dioxide and formaldehyde underline the link between wildfire emissions and increased ozone production. The comprehensive approach combining ground-based monitoring, remote sensing, and advanced modeling provides deeper insights into the dynamics of wildfire smoke and its effects on air quality, emphasizing the need for integrated strategies to manage the impacts of wildfires on regional air quality.

This study reveals wildfire smoke significantly elevated ozone levels in downwind areas, with models underestimating impacts. Integrated monitoring, remote sensing data, and modeling underscore the need for improved wildfire emission representation.

通过化学传输模型、卫星检索和内华达州农村臭氧地面观测评估野火烟雾传输的影响。
野火会将大量的臭氧前体、氮氧化物和微粒物质排放到对流层,有时甚至会排放到平流层。随着近年来野火事件的增加,美国西部地区在火灾季节(6 - 10月)可能会面临高于正常空气污染水平的挑战。因此,确定野火烟雾的臭氧增强模式对于理解野火羽流在次区域基础上的影响至关重要。本研究调查了2013年环火对内华达州农村臭氧水平的影响,采用地面监测、卫星遥感和大气模型相结合的方法。这项研究的重点是了解野火烟雾如何影响顺风地区的臭氧浓度。研究结果表明,与非烟雾日相比,烟雾日的臭氧显著增强,突出了野火排放对区域空气质量恶化的贡献。该研究表明,化学输送模型低估了野火羽流顺风处的臭氧水平,可能是由于烟雾排放估算的不确定性和不同模型版本的化学机制的差异。对二氧化氮和甲醛的卫星观测强调了野火排放与臭氧产量增加之间的联系。将地面监测、遥感和先进建模相结合的综合方法为野火烟雾的动态及其对空气质量的影响提供了更深入的见解,强调了管理野火对区域空气质量影响的综合战略的必要性。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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