A Dynamic Iterative Data Cleaning Strategy Based on Model Feedback to Enhance the Prediction Accuracy of Nanocellulose Emulsions

IF 2.1 4区 化学 Q1 SOCIAL WORK
Long Wang, Zi'ang Xia, Yao Zhang, Xiaoyu Liu, Chaojie Li, Xue Li, Jiahao Dai, Mingshun Bi, Jingxue Yang, Heng Zhang
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Abstract

The effectiveness of artificial neural networks, which were key technologies in artificial intelligence, greatly depends on the quality of the input data. Data cleaning, a crucial component of data preprocessing, played a vital role in enhancing the accuracy, robustness, and generalization capabilities of neural network models. In this study, a Feedback-Driven Iterative Cleaning (FDIC) framework, guided by model performance, was developed and applied to the study of droplet size prediction models for nanocellulose-stabilized Pickering emulsion systems. After randomly removing between 1% and 40% of the data, an artificial neural network model was established using CNC particle size (X1), CNC concentration (X2), and the oil–water volume ratio of CNC to oil-phase monomer (X3) as input variables, with emulsion droplet size (Y) as the quantitative index. The model's accuracy was evaluated after data removal using the coefficient of determination (R2), mean squared error (MSE), and mean absolute scaling error (MASE). The main finding was that targeted removal of a small portion of the data significantly improved the predictive power of the model. Specifically, removing 5% of the dataset results in optimal performance, with R2 improving from 0.5307 without cleaning to 0.7258, with an MSE of 183.4917, and MASE of 0.4060. This result suggested a significant and quantifiable improvement in the accuracy of the model through our iterative cleaning process. The study revealed a nonlinear relationship between the number of iterations and the model's generalization ability. This finding offered a novel methodological tool for data governance in the smart era and demonstrates significant value in dynamic environments.

基于模型反馈的动态迭代数据清洗策略提高纳米纤维素乳剂的预测精度
人工神经网络是人工智能的关键技术,其有效性在很大程度上取决于输入数据的质量。数据清洗是数据预处理的重要组成部分,对提高神经网络模型的准确性、鲁棒性和泛化能力起着至关重要的作用。在本研究中,以模型性能为指导,开发了一个反馈驱动迭代清洗(FDIC)框架,并将其应用于纳米纤维素稳定皮克林乳液体系的液滴尺寸预测模型的研究。随机剔除1% ~ 40%的数据后,以CNC粒度(X1)、CNC浓度(X2)、CNC与油相单体油水体积比(X3)为输入变量,以乳化液液滴粒径(Y)为定量指标,建立人工神经网络模型。剔除数据后,使用决定系数(R2)、均方误差(MSE)和平均绝对缩放误差(MASE)评估模型的准确性。主要发现是,有针对性地删除一小部分数据显著提高了模型的预测能力。具体来说,删除5%的数据集可以获得最佳性能,R2从未清理的0.5307提高到0.7258,MSE为183.4917,MASE为0.4060。这一结果表明,通过我们的迭代清洗过程,模型的准确性有了显著的、可量化的提高。研究表明,迭代次数与模型泛化能力之间存在非线性关系。这一发现为智能时代的数据治理提供了一种新的方法论工具,并在动态环境中展示了重要的价值。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
Journal of Chemometrics
Journal of Chemometrics 化学-分析化学
CiteScore
5.20
自引率
8.30%
发文量
78
审稿时长
2 months
期刊介绍: The Journal of Chemometrics is devoted to the rapid publication of original scientific papers, reviews and short communications on fundamental and applied aspects of chemometrics. It also provides a forum for the exchange of information on meetings and other news relevant to the growing community of scientists who are interested in chemometrics and its applications. Short, critical review papers are a particularly important feature of the journal, in view of the multidisciplinary readership at which it is aimed.
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