Wettability-driven pore-filling instabilities: Microfluidic and numerical insights

IF 9.4 1区 化学 Q1 CHEMISTRY, PHYSICAL
Lifei Yan , Johannes C. Müller , Tycho L. van Noorden , Bernhard Weigand , Amir Raoof
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引用次数: 0

Abstract

Hypothesis

Interface dynamics, such as Haines jumps, are crucial in multi-phase flow through porous media. However, the role of intrinsic surface wettability in pore-filling events remains unclear, and the pressure response requires further study. This work evaluates the impact of wettability on interface stability and pressure dynamics.

Experiments and simulations

We performed microfluidic experiments and level-set simulations of two-phase flow. Water displaced air or Fluorinert in a PDMS micro-model with controlled wettability (contact angles: 60, 95, 120). Three injection velocities covered capillary- to viscous-dominated flow regimes. High-resolution imaging and synchronized pressure recordings linked interface curvature with capillary pressure changes.

Findings

At low capillary numbers, wettability strongly affects burst pressure and pinning. Its influence decreases at higher capillary numbers. We observed an apparent wettability shift due to hysteresis and a capillary pressure barrier linked to pore-wall slope variations. Simulations replicated experimental trends, confirming the role of wettability in pore-scale displacement. These findings provide critical insights for improving pore-network models and understanding wettability effects in porous media.
润湿性驱动的孔隙填充不稳定性:微流体和数值见解
界面动力学,如海恩斯跳,在通过多孔介质的多相流中是至关重要的。然而,内部表面润湿性在孔隙填充事件中的作用尚不清楚,压力响应需要进一步研究。这项工作评估了润湿性对界面稳定性和压力动力学的影响。实验和模拟我们进行了微流体实验和两相流的水平集模拟。在可控制润湿性的PDMS微型模型中,水取代空气或氟化(接触角:60、95、120°)。三种注入速度涵盖了毛细管到黏度主导的流动模式。高分辨率成像和同步压力记录将界面曲率与毛细管压力变化联系起来。发现低毛细数、润湿性强烈影响破裂压力和钉住。毛细管数越高,其影响越小。我们观察到明显的润湿性变化,这是由于滞后和毛细管压力屏障与孔壁斜率变化有关。模拟重现了实验趋势,证实了润湿性在孔隙尺度驱替中的作用。这些发现为改进孔隙网络模型和理解多孔介质中的润湿性效应提供了重要见解。
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来源期刊
CiteScore
16.10
自引率
7.10%
发文量
2568
审稿时长
2 months
期刊介绍: The Journal of Colloid and Interface Science publishes original research findings on the fundamental principles of colloid and interface science, as well as innovative applications in various fields. The criteria for publication include impact, quality, novelty, and originality. Emphasis: The journal emphasizes fundamental scientific innovation within the following categories: A.Colloidal Materials and Nanomaterials B.Soft Colloidal and Self-Assembly Systems C.Adsorption, Catalysis, and Electrochemistry D.Interfacial Processes, Capillarity, and Wetting E.Biomaterials and Nanomedicine F.Energy Conversion and Storage, and Environmental Technologies
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